Synergetic Contribution of Boron and Fe-Nx Species in Porous Carbons toward Efficient Electrocatalysts for Oxygen Reduction Reaction

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期刊论文

作者：

Yuan, Kai*;Sfaelou, Stavroula;Qiu, Ming;Lutzenkirchen-Hecht, Dirk;Zhuang, Xiaodong*;...

通讯作者：

Yuan, Kai;Chen, Yiwang;Zhuang, Xiaodong

作者机构：

[Yuan, Kai; Chen, Yiwang] Nanchang Univ, Inst Polymers, Coll Chem, 999 Xuefu Ave, Nanchang 330031, Jiangxi, Peoples R China.

[Scherft, Ullrich; Yuan, Kai] Berg Univ Wuppertal, Macromol Chem Grp Buwmakro, Gauss Str 20, D-42119 Wuppertal, Germany.

[Scherft, Ullrich; Yuan, Kai] Berg Univ Wuppertal, Inst Polymer Technol, Gauss Str 20, D-42119 Wuppertal, Germany.

[Zhuang, Xiaodong; Sfaelou, Stavroula; Feng, Xinliang] Tech Univ Dresden, Cfaed, Mommsenstr 4, D-01062 Dresden, Germany.

[Zhuang, Xiaodong; Sfaelou, Stavroula; Feng, Xinliang] Tech Univ Dresden, Dept Chem & Food Chem, Mommsenstr 4, D-01062 Dresden, Germany.

通讯机构：

[Yuan, K; Chen, YW] N

[Yuan, Kai] B

[Zhuang, Xiaodong] T

Nanchang Univ, Inst Polymers, Coll Chem, 999 Xuefu Ave, Nanchang 330031, Jiangxi, Peoples R China.

Berg Univ Wuppertal, Macromol Chem Grp Buwmakro, Gauss Str 20, D-42119 Wuppertal, Germany.

语种：

英文

期刊：

ACS Energy Letters

ISSN：

2380-8195

年：

2018

卷：

期：

页码：

252-260

DOI：

10.1021/acsenergylett.7b01188

基金类别：

This work is financially supported by the National Science Fund for Distinguished Young Scholars (51425304). K.Y. thanks the financial support from the National Natural Science Foundation of China (21704038, 51763018), the Natural Science Foundation of Jiangxi Province (20171ACB21009), and the National Postdoctoral Program for Innovative Talents (BX201700112). X.Z. thanks the financial support from NSFC for Excellent Young Scholars (51722304). M.Q. thanks the support of Self-determined Research Funds of CCNU from Colleges’ Basic Research and Operation of MOE (23020205170456). The authors also thank the financial support from EU Graphene Flagship, COORNET (SPP 1928) as well as the German Science Council, Center of Advancing Electronics Dresden(cfaed).

机构署名：

本校为其他机构

院系归属：

物理科学与技术学院

摘要：

The development of porous carbon materials as highly efficient, durable, and economic electrocatalysts for oxygen reduction reaction (ORR) is of great importance for realizing practical applications of many significant energy conversion and storage devices. Herein, we demonstrate a general approach to porous carbons decorated with boron centers and atomically dispersed Fe-Nx species (denoted as FeBNC). The as-prepared FeBNC can serve as efficient electrocatalysts for ORR in an alkaline medium with a half-wave potential of 0.838 V vs RHE, compar...

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Synergetic Contribution of Boron and Fe-Nx Species in Porous Carbons toward Efficient Electrocatalysts for Oxygen Reduction Reaction

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