Air-Promoted Light-Driven Hydrogen Production from Bioethanol over Core/Shell Cr2O3@GaN Nanoarchitecture - 成果

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Air-Promoted Light-Driven Hydrogen Production from Bioethanol over Core/Shell Cr₂O₃@GaN Nanoarchitecture

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成果类型：

期刊论文

作者：

Wang, Zhouzhou;Chen, Yiqing;Sheng, Bowen;Li, Jinglin;Yao, Lin;...

通讯作者：

Zhou, BW;Song, J;Wang, XQ

作者机构：

[Zhu, Lei; Pan, Hu; Li, Jinglin; Li, Yixin; Wang, Zhouzhou; Zhou, Baowen; Yu, Tianqi; Zhou, BW] Shanghai Jiao Tong Univ, Res Ctr Renewable Synthet Fuel, Sch Mech Engn, Key Lab Power Machinery & Engn,Minist Educ, Shanghai 200240, Peoples R China.

[Wang, Zhouzhou; Yu, Ying] Cent China Normal Univ, Inst Nanosci & Nanotechnol, Coll Phys Sci & Technol, Wuhan 430079, Peoples R China.

[Song, Jun; Song, J; Chen, Yiqing] McGill Univ, Dept Min & Mat Engn, Montreal, PQ H3A0C9, Canada.

[Wang, Xinqiang; Sheng, Bowen; Wang, Ping; Wang, XQ] Peking Univ, Nanooptoelectron Frontier Ctr Minist Educ NFC MOE, Sch Phys, State Key Lab Artificial Microstruct & Mesoscop Ph, Beijing 100871, Peoples R China.

[Yao, Lin] Shanghai Jiao Tong Univ, China UK Low Carbon Coll, Shanghai 201306, Peoples R China.

通讯机构：

[Wang, XQ ] P

[Song, J ] M

[Zhou, BW ] S

Shanghai Jiao Tong Univ, Res Ctr Renewable Synthet Fuel, Sch Mech Engn, Key Lab Power Machinery & Engn,Minist Educ, Shanghai 200240, Peoples R China.

McGill Univ, Dept Min & Mat Engn, Montreal, PQ H3A0C9, Canada.

语种：

英文

关键词：

Air-promoted strategy;Photocatalytic H2 production;Bioethanol reforming;High TOF/TON;Core/shell Cr2O3@GaN nanoarchitecture

期刊：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN：

1433-7851

年：

2024

卷：

期：

页码：

e202400011-

DOI：

10.1002/anie.202400011

基金类别：

National Key Research and Development Program of China#&#&#2023YFB4004900 National Natural Science Foundation of China#&#&#No.22109095#&#&#No.62305005 Natural Science Foundation of Beijing Municipality#&#&#No.Z200004

机构署名：

本校为其他机构

院系归属：

物理科学与技术学院

摘要：

AbstractLight‐driven hydrogen production from biomass derivatives offers a path towards carbon neutrality. It is often however operated with the limitations of sluggish kinetics and severe coking. Herein, a disruptive air‐promoted strategy is explored for efficient and durable light‐driven hydrogen production from ethanol over a core/shell Cr2O3@GaN nanoarchitecture. The correlative computational and experimental investigations show ethanol is energetically favorable to be adsorbed on the Cr2O3@GaN interface, followed by dehydrogenation towa...

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Air-Promoted Light-Driven Hydrogen Production from Bioethanol over Core/Shell Cr₂O₃@GaN Nanoarchitecture

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