Flow harmonics (vn) in the Fourier expansion of the azimuthal distribution of particles are widely used to quantify the anisotropy in particle emission in high-energy heavy-ion collisions. The symmetric cumulants, SC(m,n), are used to measure the correlations between different orders of flow harmonics. These correlations are used to constrain the initial conditions and the transport properties of the medium in theoretical models. In this Letter, we present the first measurements of the four-particle symmetric cumulants in Au+Au collisions at sN...