Atomic Ni Anchored Covalent Triazine Framework as High Efficient Electrocatalyst for Carbon Dioxide Conversion

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成果类型：

期刊论文

作者：

Lu, Chenbao;Yang, Jian;Wei, Shice;Bi, Shuai;Xia, Ying;...

通讯作者：

Zhuang, Xiaodong;Hou, Yang;Qiu, Ming;Liang, Haiwei

作者机构：

[Bi, Shuai; Wei, Shice; Su, Yuezeng; Zhang, Fan; Zhuang, Xiaodong; Lu, Chenbao] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, State Key Lab Met Matrix Composites, Dongchuan Rd 800, Shanghai 200240, Peoples R China.

[Bi, Shuai; Wei, Shice; Su, Yuezeng; Zhang, Fan; Zhuang, Xiaodong; Lu, Chenbao] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai Key Lab Elect Insulat & Thermal Ageing, Dongchuan Rd 800, Shanghai 200240, Peoples R China.

[Yang, Jian; Hou, Yang] Zhejiang Univ, Minist Educ, Key Lab Biomass Chem Engn, Hangzhou 310027, Zhejiang, Peoples R China.

[Yang, Jian; Hou, Yang] Zhejiang Univ, Coll Chem & Biol Engn, Hangzhou 310027, Zhejiang, Peoples R China.

[Xia, Ying; Qiu, Ming] Cent China Normal Univ, Coll Phys Sci & Technol, Inst Nanosci & Nanotechnol, Wuhan 430079, Hubei, Peoples R China.

通讯机构：

[Zhuang, Xiaodong] S

[Hou, Yang] Z

[Qiu, Ming] C

[Liang, Haiwei] U

Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, State Key Lab Met Matrix Composites, Dongchuan Rd 800, Shanghai 200240, Peoples R China.

语种：

英文

关键词：

carbon dioxide reduction;covalent triazine framework;energy barrier;Faradaic efficiency;nickel–nitrogen coordination

期刊：

Advanced Functional Materials

ISSN：

1616-301X

年：

2019

卷：

期：

页码：

1806884-

DOI：

10.1002/adfm.201806884

基金类别：

C.L. and J.Y. contributed equally to this work. This work was financially supported by National Natural Science Foundation of China for Excellent Young Scholars (51722304), National Natural Science Foundation of China (21720102002 and 5171101862), Shanghai Committee of Science and Technology (16JC1400703), Shanghai Pujiang Talent Program (18PJ1406100), and Open Project Program of the State Key Laboratory of Photocatalysis on Energy and Environment (SKLPEE-KF201702, Fuzhou University). Y.H. thanks the support of NSFC 51702284 and 21878270. M.Q. thanks the support of Hubei Natural Science Foundation of China (2018CFB531) and Self-Determined Research Funds of CCNU from Colleges’ Basic Research and Operation of MOE (CCNU18TS048).

机构署名：

本校为通讯机构

院系归属：

物理科学与技术学院

摘要：

Electrochemically driven carbon dioxide (CO 2 ) conversion is an emerging research field due to the global warming and energy crisis. Carbon monoxide (CO) is one key product during electroreduction of CO 2 ; however, this reduction process suffers from tardy kinetics due to low local concentration of CO 2 on a catalyst's surface and low density of active sites. Herein, presented is a combination of experimental and theoretical validation of a Ni porphyrin-based covalent triazine framework (NiPor-CTF) with atomically dispersed NiN 4 centers as a...

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Atomic Ni Anchored Covalent Triazine Framework as High Efficient Electrocatalyst for Carbon Dioxide Conversion

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