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Oxygen Vacancy-Mediated Photocatalysis of BiOCl: Reactivity, Selectivity, and Perspectives

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成果类型:
期刊论文
作者:
Li, Hao;Li, Jie;Ai, Zhihui;Jia, Falong;Zhang, Lizhi*
通讯作者:
Zhang, Lizhi
作者机构:
[Zhang, Lizhi; Li, Hao; Li, Jie; Ai, Zhihui; Jia, Falong] Cent China Normal Univ, Coll Chem, Inst Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Hubei, Peoples R China.
通讯机构:
[Zhang, Lizhi] C
Cent China Normal Univ, Coll Chem, Inst Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Hubei, Peoples R China.
语种:
英文
关键词:
BiOCl;nitrogen fixation;oxygen activation;photocatalysis;water splitting
期刊:
Angewandte Chemie - International Edition
ISSN:
1433-7851
年:
2018
卷:
57
期:
1
页码:
122-138
基金类别:
We thank all of our co-workers, whose names appear in the related references, for their significant contributions to this review. This work was supported by the National Key Research and Development Program of China (Grant 2016YFA0203002), National Natural Science Funds for Distinguished Young Scholars (Grant 21425728), the National Basic Research Program of China (973 Program) (Grant 2013CB632402), the National Science Foundation of China (Grant 51472100), and an Excellent Doctoral Dissertation Cultivation Grant from the Central China Normal University (Grant 2015YBZD018 and 2016YBZZ034).
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
Semiconductor photocatalysis is a trustworthy approach to harvest clean solar light for energy conversions, while state-of-the-art catalytic efficiencies are unsatisfactory because of the finite light response and/or recombination of robust charge carriers. Along with the development of modern material characterization techniques and electronic-structure computations, oxygen vacancies (OVs) on the surface of real photocatalysts, even in infinitesimal concentration, are found to play a more decisive role in determining the kinetics, energetics, ...

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