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Acid-Mediated Intermolecular [3 + 2] Cycloaddition toward Pyrrolo[2,1‑a]isoquinolines: Total Synthesis of the Lamellarin Core and Lamellarin G Trimethyl Ether

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成果类型:
期刊论文
作者:
Zheng, Kai-Lu;You, Min-Qi;Shu, Wen-Ming;Wu, Yan-Dong*;Wu, An-Xin*吴安心
通讯作者:
Wu, Yan-Dong;Wu, An-Xin(吴安心
作者机构:
[Wu, An-Xin; Wu, Yan-Dong; Zheng, Kai-Lu; You, Min-Qi; Shu, Wen-Ming] Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Hubei, Peoples R China.
通讯机构:
[Wu, YD; Wu, AX] C
Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Hubei, Peoples R China.
语种:
英文
期刊:
Organic Letters
ISSN:
1523-7060
年:
2017
卷:
19
期:
9
页码:
2262-2265
基金类别:
National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21602070, 21472056]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [CCNU15ZX002, CCNU16A05002]; Central China Normal University [2016CXZZ64]; 111 ProjectMinistry of Education, China - 111 Project [B17109]
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
A novel one-pot reaction has been developed for the efficient synthesis of pyrrolo[2,1-a]isoquinolines and 1-dearyllamellarin core from (E)-(2-nitrovinyl)benzenes and azomethine ylides generated in situ. This strategy provides a concise total synthesis of the lamellarin core and lamellarin G trimethyl ether using electrophilic substitution and palladium-ca...

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