期刊论文

Zhang, Lizhi;Ling, Lan

英文

Environmental Science: Nano

2051-8153

2019

6

3

892-903

10.1039/c8en00899j

This work was supported by the Natural Science Funds for Distinguished Young Scholars (Grant 21425728), the National Science Foundation of China (Grant 21677059 and 21677107), the 111 Project (Grant B17019), and the CAS Interdisciplinary Innovation Team of the Chinese Academy of Sciences. We also acknowledge beam line 1W1B of BSRF for the EXAFS measurements and the National Supercomputer Center in Ji-nan for the high performance computation. We greatly acknowledge the four anonymous reviewers who helped to improve the quality of the manuscript.

本校为第一且通讯机构

As the fate, transport and bioavailability of U(vi) in subsurface environments are strongly influenced by its adsorption structures on iron minerals such as hematite, we systematically studied the molecular-scale structures of U(vi) complexes formed at the interfaces of hematite and water with periodic density-functional theory (DFT) calculation, extended X-ray absorption fine structure (EXAFS) measurements, attenuated total reflectance Fourier transform infrared (ATR-FTIR) spectroscopy, and spherical aberration-corrected scanning transmission ...