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Visible-Light-Induced Decarboxylative Functionalization of Carboxylic Acids and Their Derivatives

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成果类型:
期刊论文
作者:
Xuan, Jun;Zhang, Zhao-Guo*;Xiao, Wen-Jing
通讯作者:
Zhang, Zhao-Guo
作者机构:
[Xiao, Wen-Jing; Xuan, Jun] Cent China Normal Univ, Coll Chem, Minist Educ, CCNU uOttawa Joint Res Ctr,Key Lab Pesticide & Ch, Wuhan 430079, Hubei, Peoples R China.
[Zhang, Zhao-Guo] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China.
[Zhang, Zhao-Guo] Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, 800 Dongchuan Rd, Shanghai 200240, Peoples R China.
通讯机构:
[Zhang, Zhao-Guo] S
Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, 800 Dongchuan Rd, Shanghai 200240, Peoples R China.
语种:
英文
关键词:
C?C coupling;carboxylic acids;photochemistry;radicals;synthetic methods
期刊:
Angewandte Chemie - International Edition
ISSN:
1433-7851
年:
2015
卷:
54
期:
52
页码:
15632-15641
基金类别:
National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21232003, 21202053, 21272087, 21472057]; National Basic Research Program of ChinaNational Basic Research Program of China [2011CB808603]
机构署名:
本校为第一机构
院系归属:
化学学院
摘要:
Visible-light-induced radical decarboxylative functionalization of carboxylic acids and their derivatives has recently received considerable attention as a novel and efficient method to create C-C and C-X bonds. Generally, this visible-light-promoted decarboxylation process can smoothly occur under mild reaction conditions with a broad range of substrates and an excellent functional-group tolerance. The radical species formed from the decarboxylation step can participate in not only single photocatalytic transformations, but also dual-catalytic...

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