Boosting Oxygen Reduction of Single Iron Active Sites via Geometric and Electronic Engineering: Nitrogen and Phosphorus Dual Coordination

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成果类型：

期刊论文

作者：

Yuan, Kai*;Luetzenkirchen-Hecht, Dirk;Li, Longbin;Shuai, Ling;Li, Yizhe;...

通讯作者：

Yuan, Kai;Chen, Yiwang;Qiu, Ming;Zhuang, Xiaodong

作者机构：

[Yuan, Kai; Chen, Yiwang; Li, Longbin; Li, Yizhe] Nanchang Univ, Inst Polymers & Energy Chem, Coll Chem, 999 Xuefu Ave, Nanchang 330031, Jiangxi, Peoples R China.

[Yuan, Kai; Scherf, Ullrich] Berg Univ Wuppertal, Macromol Chem Grp Buwmakro, Gauss Str 20, D-42119 Wuppertal, Germany.

[Luetzenkirchen-Hecht, Dirk; Yuan, Kai; Scherf, Ullrich] Berg Univ Wuppertal, Inst Polymer Technol, Gauss Str 20, D-42119 Wuppertal, Germany.

[Shuai, Ling; Qiu, Ming] Cent China Normal Univ, Coll Phys Sci & Technol, Inst Nanosci & Nanotechnol, Wuhan 430079, Peoples R China.

[Zhuang, Xiaodong] Shanghai Jiao Tong Univ, Shanghai Key Lab Elect Insulat & Thermal Ageing, State Key Lab Met Matrix Composites, Sch Chem & Chem Engn,Soft2D Lab, Dongchuan Rd 800, Shanghai 200240, Peoples R China.

通讯机构：

[Yuan, K; Chen, YW] N

[Yuan, Kai] B

[Qiu, Ming] C

[Zhuang, Xiaodong] S

Nanchang Univ, Inst Polymers & Energy Chem, Coll Chem, 999 Xuefu Ave, Nanchang 330031, Jiangxi, Peoples R China.

语种：

英文

期刊：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

ISSN：

0002-7863

年：

2020

卷：

142

期：

页码：

2404-2412

DOI：

10.1021/jacs.9b11852

基金类别：

K.Y. is grateful for the financial support from NSFC (21704038, 51763018), China Postdoctoral Science Foundation (2018M632599), National Postdoctoral Program for Innovative Talents (BX201700112), Natural Science Foundation of Jiangxi Province (20192BCB23001, 2018ACB21021, 20171ACB21009). Y.C. is grateful for the financial support from NSFC-DFG Joint Research Project (51761135114). X.Z. is grateful for the financial support from National Key Research and Development Program of China (2017YFE9134000), NSFC Excellent Young Scientists Fund (51722304), NSFC (51811530013, 51973114, 21720102002), Shanghai Pujiang Talent Program (18PJ1406100), and SMSTC (19JC412600). M.Q. is grateful for the support of Hubei Natural Science Foundation of China (2018CFB531) and Self-determined Research Funds of CCNU from Colleges’ Basic Research and Operation of MOE (CCNU18TS045).

机构署名：

本校为通讯机构

院系归属：

物理科学与技术学院

摘要：

Atomically dispersed transition metal active sites have emerged as one of the most important fields of study because they display promising performance in catalysis and have the potential to serve as ideal models for fundamental understanding. However, both the preparation and determination of such active sites remain a challenge. The structural engineering of carbon- and nitrogen-coordinated metal sites (M-N-C, M = Fe, Co, Ni, Mn, Cu, etc.) via employing new heteroatoms, e.g., P and S, remains challenging. In this study, carbon nanosheets embe...

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Boosting Oxygen Reduction of Single Iron Active Sites via Geometric and Electronic Engineering: Nitrogen and Phosphorus Dual Coordination

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