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Efficient electroreduction of CO2 on bulk silver electrode in aqueous solution via the inhibition of hydrogen evolution

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成果类型:
期刊论文
作者:
Quan, Fengjiao;Xiong, Mubing;Jia, Falong*;Zhang, Lizhi
通讯作者:
Jia, Falong
作者机构:
[Quan, Fengjiao; Zhang, Lizhi; Xiong, Mubing; Jia, Falong] Cent China Normal Univ, Inst Environm Chem, Coll Chem, Wuhan 430079, Peoples R China.
通讯机构:
[Jia, Falong] C
Cent China Normal Univ, Inst Environm Chem, Coll Chem, Wuhan 430079, Peoples R China.
语种:
英文
关键词:
Carbon dioxide;Electrocatalytic reduction;Hydrogen evolution;Silver electrode
期刊:
Applied Surface Science
ISSN:
0169-4332
年:
2017
卷:
399
页码:
48-54
基金类别:
self-determined research funds of CCNU from the colleges' basic research and operation of MOE [CCNU15A02010]
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
Electrochemical CO 2 reduction provides a desirable pathway to convert greenhouse gas into useful chemicals. It is a great challenge to reduce CO 2 efficiently in aqueous solution, especially on commercial bulk metal electrodes. Here, we report substantial improvement in CO 2 reduction on bulk silver electrode through the introduction of ionic surfactant in aqueous electrolyte. The hydrogen evolution on the electrode surface is greatly suppressed by the surfactant, while the catalytic ability of silver towards CO 2 reduction is maintained. The ...

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