Amorphization enables highly efficient anaerobic thiamphenicol reduction by zero-valent iron

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成果类型：

期刊论文

作者：

Shen, Wenjuan;Wang, Xiaoming;Jia, Falong*;Tong, Zhe;Sun, Hongwei;...

通讯作者：

Jia, Falong;Ai, Zhihui;Zhang, Lizhi

作者机构：

[Zhang, Lizhi; Jia, FL; Ai, ZH; Zhang, LZ; Sun, Hongwei; Wang, Xiaobing; Shen, Wenjuan; Jia, Falong; Tong, Zhe; Song, Fahui; Ai, Zhihui] Cent China Normal Univ, Inst Environm & Appl Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.

[Wang, Xiaoming] Huazhong Agr Univ, Minist Agr, Coll Resources & Environm, Key Lab Arable Land Conservat Middle & Lower Reac, Wuhan 430070, Peoples R China.

[Chai, Bo; Shen, Wenjuan] Wuhan Polytech Univ, Sch Chem & Environm Engn, Wuhan 430023, Peoples R China.

通讯机构：

[Jia, FL; Ai, ZH; Zhang, LZ] C

Cent China Normal Univ, Inst Environm & Appl Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.

语种：

英文

关键词：

Amorphous zero-valent iron;Anaerobic reduction;Ethylenediamine;Formation mechanism;Thiamphenicol

期刊：

Applied Catalysis B: Environmental

ISSN：

0926-3373

年：

2020

卷：

264

页码：

118550

DOI：

10.1016/j.apcatb.2019.118550

基金类别：

National Key Research and Development Program of China [2018YFC1800801, 2016YFA0203000]; Natural Science Funds for Distinguished Young ScholarsNational Natural Science Foundation of ChinaNational Science Fund for Distinguished Young Scholars [21425728]; National Science Foundation of ChinaNational Natural Science Foundation of China [21906126, 21936003, 21876058, 21777050, 41601543]; 111 ProjectMinistry of Education, China - 111 Project [B17019]; Self-Determined Research Funds of CCNU from the Colleges' Basic Research and Operation of MOE [CCNU16A04005]

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

As a new member of zero-valent iron (ZVI) family, amorphous zero-valent iron microspheres (A-mZVI) were very promising for the aerobic disinfection of Escherichia coli. However, their formation and anaerobic reduction performance are still unknown. In this study, we investigated A-mZVI's formation mechanism and checked its anaerobic reduction ability with using thiamphenicol as a model contaminant, and found that the presence of ethylenediamine decreased the reducing capacity of NaBH4, the Fe(II) reduction rate, and the energy for crystal growt...

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Amorphization enables highly efficient anaerobic thiamphenicol reduction by zero-valent iron

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