Temperature-Dependent Tunneling in Furan Oligomer Single-Molecule Junctions

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期刊论文

作者：

Li, Haipeng B.;Xi, Yan-Feng;Hong, Ze-Wen;Yu, Jingxian;Li, Xiao-Xia;...

通讯作者：

Jin, S.;Hihath, J.;Zhou, X.-S.

作者机构：

[Xi, Yan-Feng; Jin, Shan; Li, Xiao-Xia; Liu, Wen-Xia; Li, Haipeng B.] Cent China Normal Univ, Coll Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.

[Hihath, Joshua; Domulevicz, Lucas; Li, Haipeng B.] Univ Calif Davis, Dept Elect & Comp Engn, Davis, CA 95616 USA.

[Zhou, Xiao-Shun; Hong, Ze-Wen] Zhejiang Normal Univ, Inst Phys Chem, Zhejiang Key Lab React Chem Solid Surfaces, Jinhua 321004, Zhejiang, Peoples R China.

[Yu, Jingxian] Univ Adelaide, ARC Ctr Excellence Nanoscale BioPhoton CNBP, Inst Photon & Adv Sensing, Dept Chem, Adelaide, SA 5005, Australia.

通讯机构：

[Shan Jin] K

[Xiao-Shun Zhou] Z

[Joshua Hihath] D

Key Laboratory of Pesticide and Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, Wuhan 430079, China<&wdkj&>Zhejiang Key Laboratory for Reactive Chemistry on Solid Surfaces, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, Zhejiang 321004, China<&wdkj&>Department of Electrical and Computer Engineering, University of California Davis, Davis, California 95616, United States

语种：

英文

关键词：

molecular electronics;charge transport;thermally assisted tunneling;furan-based molecular wire;single-molecular conductance;single-molecule break junction

期刊：

ACS SENSORS

ISSN：

2379-3694

年：

2021

卷：

期：

页码：

565-572

DOI：

10.1021/acssensors.0c02278

基金类别：

National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21573086, 21573198, 21872062, 21872126, 22072053]; Australian Research CouncilAustralian Research Council [CE140100003, DP180101581]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [CCNU19TS008]; U.S. National Science FoundationNational Science Foundation (NSF) [ECCS1807555]

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

Two commonly observed charge transport mechanisms in single-molecule junctions are coherent tunneling and incoherent hopping. It has been generally believed that tunneling processes yield temperature-independent conductance behavior and hopping processes exhibit increasing conductance with increasing temperature. However, it has recently been proposed that tunneling can also yield temperature-dependent transport due to the thermal broadening of the Fermi energy of the contacts. In this work, we examine a series of rigid, planar furan oligomers ...

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Temperature-Dependent Tunneling in Furan Oligomer Single-Molecule Junctions

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