High-order dipolar annulations with metal-containing reactive dipoles

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成果类型：

期刊论文

作者：

Zhang, Mao-Mao;Qu, Bao-Le;Shi, Bin;Xiao, Wen-Jing;Lu, Liang-Qiu

通讯作者：

Lu, LQ

作者机构：

[Lu, Liang-Qiu; Lu, LQ; Qu, Bao-Le; Xiao, Wen-Jing; Zhang, Mao-Mao; Shi, Bin] Cent China Normal Univ, Coll Chem, CCNU uOttawa Joint Res Ctr, Key Lab Pesticide & Chem Biol,Minist Educ, 152 Luoyu Rd, Wuhan 430079, Peoples R China.

[Xiao, Wen-Jing] Shanghai Inst Organ Chem, State Key Lab Organometall Chem, 345 Lingling Rd, Shanghai 200032, Peoples R China.

[Lu, Liang-Qiu; Lu, LQ] Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Oxo Synth & Select Oxidat, Lanzhou 730000, Peoples R China.

[Lu, Liang-Qiu; Lu, LQ] Henan Normal Univ, Sch Chem & Chem Engn, Xinxiang 453007, Henan, Peoples R China.

通讯机构：

[Lu, LQ ] C

Cent China Normal Univ, Coll Chem, CCNU uOttawa Joint Res Ctr, Key Lab Pesticide & Chem Biol,Minist Educ, 152 Luoyu Rd, Wuhan 430079, Peoples R China.

Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Oxo Synth & Select Oxidat, Lanzhou 730000, Peoples R China.

Henan Normal Univ, Sch Chem & Chem Engn, Xinxiang 453007, Henan, Peoples R China.

语种：

英文

期刊：

CHEMICAL SOCIETY REVIEWS

ISSN：

0306-0012

年：

2022

卷：

期：

页码：

4146-4174

DOI：

10.1039/d1cs00897h

基金类别：

National Science Foundation of China [21822103, 21820102003, 21772052, 21772053, 91956201]; Program of Introducing Talents of Discipline to Universities of China (111 Program) [B17019]; Natural Science Foundation of Hubei Province [2017AHB047]; International Joint Research Center for Intelligent Biosensing Technology and Health

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

Medium-sized heterocycles are widespread among a spectrum of structurally intriguing and biologically significant natural products and synthetic pharmaceuticals. Metal-catalyzed high-order dipolar annulations resembling reactions of metal-containing reactive dipoles with dipolarophiles constitute a highly efficient and flexible strategy for constructing medium-sized heterocycles. Mechanistically, these annulation reactions usually proceeding through stepwise pathways are different from the classic high-order pericyclic reactions that follow the...

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High-order dipolar annulations with metal-containing reactive dipoles

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