Mn2+ promoted Cr(VI) reduction with oxalic acid: The indispensable role of In-situ generated Mn3+

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成果类型：

期刊论文

作者：

Mu, Yi;Jiang, Xu;Ai, Zhihui*;Jia, Falong;Zhang, Lizhi*

通讯作者：

Ai, Zhihui;Zhang, Lizhi

作者机构：

[Zhang, Lizhi; Mu, Yi; Jiang, Xu; Ai, ZH; Zhang, LZ; Ai, Zhihui; Jia, Falong] Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Inst Environm & Appl Chem,Coll Chem, Wuhan 430079, Hubei, Peoples R China.

通讯机构：

[Ai, ZH; Zhang, LZ] C

Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Inst Environm & Appl Chem,Coll Chem, Wuhan 430079, Hubei, Peoples R China.

语种：

英文

关键词：

In situ processing;Manganese;Manganese removal (water treatment);Organic acids;Oxalic acid;Rate constants;Acceleration process;Acid wastewater;Cr reductions;Electron transfer;Induction periods;Initial induction;Natural aquatic environments;Ternary complex;Chromium compounds;chromium;manganese;oxalic acid;aquatic environment;cation;chromium;electron;in situ measurement;oxalic acid;oxidation;pH;reduction;transformation;wastewater;wastewater treatment;acceleration;aquatic environment;Article;automation;bioremediation;biotransformation;chemical analysis;comparative study;concentration (parameters);controlled study;electron transport;metal recovery;oxidation;oxidation reduction reaction;proton transport;rate constant;reaction time;waste water management

期刊：

Journal of Hazardous Materials

ISSN：

0304-3894

年：

2018

卷：

343

页码：

356-363

DOI：

10.1016/j.jhazmat.2017.10.008

基金类别：

This work was supported by Natural Science Funds for The National Key Research and Development Program of China ( 2016YFA0203000 ), Distinguished Young Scholars (Grant 21425728 ), National Science Foundation of China (Grant 21177048 , 21173093 , 21477044 , and 51472100 ), Self−Determined Research Funds of CCNU from the Colleges’ Basic Research and Operation of MOE (Grant CCNU16A02029 , CCNU16A04005 , CCNU14Z01001 , and CCNU14KFY002 ), the 111 Project (Grant B17019), and Excellent Doctorial Dissertation Cultivation Grant from Central China Normal University ( 2015YBZD024 and 2016YBZZ031 ).

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

In this study, we demonstrate that Mn(2+) can greatly promote the Cr(VI) reduction by oxalic acid at pH

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Mn2+ promoted Cr(VI) reduction with oxalic acid: The indispensable role of In-situ generated Mn3+

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