Construction of Pillar[5]arene-based Nanochannels with Chiral-enhanced DNA Translocation Ability

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成果类型：

期刊论文

作者：

Yang, Lei;Zhang, Fan;Quan, Jiaxin;Li, Jia;Li, Haibing

通讯作者：

Li, Haibing(lhbing@mail.ccnu.edu.cn);Li, Jia(2014079@mail.scuec.edu.cn)

作者机构：

[Yang, Lei; Li, Haibing] Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol CCNU, Wuhan 430079, Peoples R China.

[Zhang, Fan] Hubei Univ, Hubei Collaborat Innovat Ctr Adv Organ Chem Mat, Minist Educ, Key Lab Synth & Applicat Organ Funct Mol,Coll Che, Wuhan 430062, Peoples R China.

[Quan, Jiaxin] Hanjiang Normal Univ, Coll Chem & Environm Engn, Shi Yan 432200, Peoples R China.

[Li, Jia] South Cent Minzu Univ, Coll Resources & Environm Sci, Wuhan 430074, Peoples R China.

通讯机构：

[Prof. Jia Li; Prof. Jia Li Prof. Jia Li Prof. Jia Li] C

[Prof. Dr. Haibing Li; Prof. Dr. Haibing Li Prof. Dr. Haibing Li Prof. Dr. Haibing Li] K

Key Laboratory of Pesticide and Chemical Biology (CCNU) Ministry of Education, College of Chemistry, Central China Normal University, Wuhan, 430079 P. R. China<&wdkj&>College of Resources and Environmental Science, South-Central Minzu University, Wuhan, 430074 P. R. China

语种：

英文

关键词：

DANN;multi-chiral;nanochannel;pillar[5]arene;translocation

期刊：

ChemNanoMat

ISSN：

2199-692X

年：

2022

卷：

期：

页码：

e202200342-

DOI：

10.1002/cnma.202200342

基金类别：

H.B. Li and J. Li is thankful for the Key R&D Projects of Hubei Province (2022BCA061), the National Key Research and Development Program (2021YFA0716702), the National Natural Science Foundation of China (22071074, 21772055), the 111 Project (B17019) and Self‐determined research funds of CCNU from the colleges’ basic research and operation of MOE.

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

Chirality is an intrinsic feature of nature and plays a crucial role in molecular translocation. However, how chirality affects or even more strongly affects DNA translocation remains largely unknown. Here, a facile and feasible strategy was contributed for the construction of chiral pillar[5]arene-modified nanochannels (D/L-Phe-P5 nanochannels) that can enhance recognition and accelerate DNA translocation. The results showed the L-Phe-P5 nanochannel elevated the DNA translocation efficiency by about 6.59-fold compared to the Mono-L-Phe-P5 chan...

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Construction of Pillar[5]arene-based Nanochannels with Chiral-enhanced DNA Translocation Ability

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