Hydrothermal Carbon-Mediated Fenton-Like Reaction Mechanism in the Degradation of Alachlor: Direct Electron Transfer from Hydrothermal Carbon to Fe(III)

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成果类型：

期刊论文

作者：

Qin, Yaxin;Zhang, Lizhi*;An, Taicheng*

通讯作者：

An, Taicheng;Zhang, Lizhi

作者机构：

[An, Taicheng; Qin, Yaxin] Guangdong Univ Technol, Sch Environm Sci & Engn, Inst Environm Hlth & Pollut Control, Guangzhou Key Lab Environm Catalysis & Pollut Con, Guangzhou 510006, Guangdong, Peoples R China.

[Zhang, Lizhi; Qin, Yaxin] Cent China Normal Univ, Coll Chem, Inst Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

通讯机构：

[An, Taicheng] G

[Zhang, Lizhi] C

Guangdong Univ Technol, Sch Environm Sci & Engn, Inst Environm Hlth & Pollut Control, Guangzhou Key Lab Environm Catalysis & Pollut Con, Guangzhou 510006, Guangdong, Peoples R China.

Cent China Normal Univ, Coll Chem, Inst Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

语种：

英文

关键词：

hydrothermal carbon;fenton-like reaction;Fe(III)/Fe(II) cycle;electron transfer mechanism;alachlor degradation

期刊：

ACS Applied Materials & Interfaces

ISSN：

1944-8244

年：

2017

卷：

期：

页码：

17115-17124

DOI：

10.1021/acsami.7b03310

基金类别：

National Natural Science Funds for Distinguished Young ScholarsNational Natural Science Foundation of China (NSFC)National Science Fund for Distinguished Young Scholars [21425728, 41425015]; National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21273088, 21477044]; Self-Determined Research Funds of CCNU from the Colleges' Basic Research and Operation of MOE [CCNU14Z01001, CCNU14K-FY002]

机构署名：

本校为通讯机构

院系归属：

化学学院

摘要：

As Fenton systems suffer from the undesirable Fe(III)/Fe(II) cycle, great efforts were made to realize the effective reduction of Fe(III) to Fe(II). The effects of hydrothermal carbon (HTC) on the Fe(III)/H2O2Fenton-like reaction and the subsequent degradation of alachlor in water was systematically investigated, and the results indicated that HTC could enhance alachlor degradation in Fe(III)/H2O2by promoting the Fe(III)/Fe(II) cycle via electron transfer from HTC to Fe(III) ions. The apparent alachlor degradation rate constant in the HTC-G/Fe(III)/H2O2system (7.02 ×10-2min-1) was about ...

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Hydrothermal Carbon-Mediated Fenton-Like Reaction Mechanism in the Degradation of Alachlor: Direct Electron Transfer from Hydrothermal Carbon to Fe(III)

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