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Dual-site activation enhanced photocatalytic removal of no with Au/CeO2

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成果类型:
期刊论文
作者:
Shang, Huan;Huang, Shun;Li, Hao;Li, Meiqi;Zhao, Shengxi;...
通讯作者:
Ai, Zhihui;Zhang, Lizhi
作者机构:
[Wang, Jiaxian; Zhang, Lizhi; Shang, Huan; Li, Hao; Ai, ZH; Zhang, LZ; Zhao, Shengxi; Huang, Shun; Ai, Zhihui; Li, Meiqi] Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Inst Environm & Appl Chem, Wuhan 430079, Peoples R China.
通讯机构:
[Ai, ZH; Zhang, LZ] C
Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Inst Environm & Appl Chem, Wuhan 430079, Peoples R China.
语种:
英文
关键词:
Air purification;Dual-site activation;Oxygen vacancy;Photocatalytic NO removal
期刊:
Chemical Engineering Journal
ISSN:
1385-8947
年:
2020
卷:
386
页码:
124047
基金类别:
National Key Research and Development Program of China [2016YFA0203000]; Natural Science Funds for Distinguished Young ScholarsNational Natural Science Foundation of China (NSFC)National Science Fund for Distinguished Young Scholars [21425728]; National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21876058, 21477044]; 111 ProjectMinistry of Education, China - 111 Project [B17019]
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
Photocatalytic technology provides an effective strategy for aerobic purification of dilute gaseous NO pollutant, but suffers from its low efficiency. In this study, we demonstrate that the bicomponent Au/CeO2 photocatalyst possesses an enhanced photocatalytic NO removal performance under visible light irradiation, with a higher NO conversion efficiency (65%) and triple rate constant (0.1451 min−1) versus CeO2 (50%, 0.0448 min−1). Density function theory calculations and experimental results revealed that oxygen vacancies on the CeO2 componen...

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