Pd Metallene Aerogels with Single-Atom W Doping for Selective Ethanol Oxidation

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成果类型：

期刊论文

作者：

Wang, Hengjia;Zheng, Huiling;Ling, Ling;Fang, Qie;Jiao, Lei;...

通讯作者：

Zhu, Chengzhou(czzhu@ccnu.edu.cn);Song, Weiyu(songwy@cup.edu.cn)

作者机构：

[Fang, Qie; Qin, Ying; Luo, Zhen; Zhu, Chengzhou; Jiao, Lei; Gu, Wenling; Wang, Hengjia; Ling, Ling] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Key Lab Pesticides & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

[Zheng, Huiling] Taiyuan Univ Technol, State Key Lab Clean & Efficient Coal Utilizat, Taiyuan 030024, Peoples R China.

[Zheng, Lirong] Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China.

[Song, Weiyu] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China.

通讯机构：

[Weiyu Song] S

[Chengzhou Zhu] K

State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing 102249, P. R. China<&wdkj&>Key Laboratory of Pesticides and Chemical Biology of Ministry of Education, International Joint Research Center for Intelligent Biosensing Technology and Health, College of Chemistry, Central China Normal University, Wuhan 430079, P. R. China

语种：

英文

关键词：

aerogels;metallene;single-atom doping;ethanol oxidation reaction;electrocatalysis

期刊：

ACS Nano

ISSN：

1936-0851

年：

2022

卷：

期：

页码：

21266-21274

DOI：

10.1021/acsnano.2c09270

基金类别：

National Key R & D Program of China [2021YFC2901100]; Fundamental Research Funds for the Central Universities [CCNU20TS013, CCNU20QN007]; Program of Introducing Talents of Discipline to Universities of China (111 program) [B17019]; Fundamental Research Funds for the Central Universities (Youbo Cultivation Project) [2022YBZZ005]

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

The development of advanced electrocatalysts with satisfactory C1 pathway selectivity for the ethanol oxidation reaction (EOR) is critical. Herein, a bubbling CO-induced gelation method is developed in acetic acid at 50 °C to construct single-atom W-doped Pd metallene aerogels (denoted as SA W-Pd MAs) within 1 h. In light of the metallene structural advantages of noble metal aerogels and single-atom W decoration, the resultant SA W-Pd MAs exhibit an outstanding EOR performance with high C1 pathway selectivity. Density functional theory calcula...

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Pd Metallene Aerogels with Single-Atom W Doping for Selective Ethanol Oxidation

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