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Cascade Reaction System Integrating Single-Atom Nanozymes with Abundant Cu Sites for Enhanced Biosensing

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成果类型:
期刊论文
作者:
Wu, Yu;Wu, Jiabin;Jiao, Lei;Xu, Weiqing;Wang, Hengjia;...
通讯作者:
Huang, Liang;Zhu, Chengzhou
作者机构:
[Zhu, Chengzhou; Jiao, Lei; Gu, Wenling; Xu, Weiqing; Wu, Yu; Wei, Xiaoqian; Wang, Hengjia] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol, Key Lab Pesticides & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
[Huang, Liang; Wu, Jiabin] Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430074, Peoples R China.
[Zhang, Nian; Ren, Guoxi] Chinese Acad Sci, SIMIT, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China.
[Zhang, Qinghua; Gu, Lin] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.
[Zhang, Qinghua; Gu, Lin] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.
通讯机构:
[Huang, Liang] H
[Zhu, Chengzhou] C
Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430074, Peoples R China.
Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol, Key Lab Pesticides & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
语种:
英文
期刊:
Analytical Chemistry
ISSN:
0003-2700
年:
2020
卷:
92
期:
4
页码:
3373-3379
基金类别:
The authors gratefully acknowledge the financial support of the Fundamental Research Funds for the Central Universities (CCNU19QN066), the National Natural Science Foundation of China (Grants 51602115, 51902115, and 51972124), the Program of Introducing Talents of Discipline to Universities of China (111 program, B17019), and the Recruitment Program of Global Youth Experts of China. The authors thank the facility support of the Center for Nanoscale Characterization & Devices, WNLO-HUST, and the Analysis and Testing Center, HUST.
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
Single-atom nanozymes (SAzymes), as novel nanozymes with atomically dispersed active sites, are of great importance in the development of nanozymes for their high catalytic activities, the maximum utilization efficiency of metal atoms, and the simple model of active sites. Herein, the peroxidase-like SAzymes with high-concentration Cu sites on carbon nanosheets (Cu-N-C) were synthesized through a salt-template strategy. With the densely distributed active Cu atoms (â¼5.1 wt %), the Cu-N-C SAzymes exhibit remarkable activity to mimic natural p...

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