Iridium Single-Atomic Site Catalysts with Superior Oxygen Reduction Reaction Activity for Sensitive Monitoring of Organophosphorus Pesticides

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成果类型：

期刊论文

作者：

Luo, Xin;Luo, Zhen;Wei, Xiaoqian;Jiao, Lei;Fang, Qie;...

通讯作者：

Zhu, CZ

作者机构：

[Luo, Zhen; Fang, Qie; Zhu, Chengzhou; Wei, Xiaoqian; Jiao, Lei; Zhu, CZ; Luo, Xin; Gu, Wenling; Wang, Hengjia] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

[Wang, Jinhua; Luo, Xin] Hubei Univ Technol, Hubei Res Ctr Food Fermentat Engn & Technol, Minist Educ,Natl 111 Ctr Cellular Regulat & Mol P, Hubei Prov Cooperat Innovat Ctr Ind Fermentat,Key, Wuhan 430068, Peoples R China.

[Hu, Liuyong] Wuhan Inst Technol, Sch Mat Sci & Engn, Hubei Key Lab Plasma Chem & Adv Mat, Wuhan 430205, Peoples R China.

通讯机构：

[Zhu, CZ ] C

Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

语种：

英文

期刊：

Analytical Chemistry

ISSN：

0003-2700

年：

2022

卷：

期：

页码：

1390-1396

DOI：

10.1021/acs.analchem.1c04665

基金类别：

National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [22074049, 22104114, 22004042]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [CCNU20QN007, CCNU20TS013]; Program of Introducing Talents of Discipline to Universities of China (111 program) [B17019]

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

Tremendous efforts have been made in developing single-atomic site catalysts (SASCs) for oxygen reduction reaction (ORR), which is regarded as a pivotal cornerstone in electrochemical energy conversion. However, SASCs for ORR have not been explored for electrochemical sensing. Herein, a template-sacrificed strategy is reported for the synthesis of atomically dispersed Ir SASCs, serving as a sensing platform to detect organophosphorus pesticides (OPs) with high sensitivity and selectivity. Owing to abundant Ir single-atom active sites, Ir SASCs ...

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Iridium Single-Atomic Site Catalysts with Superior Oxygen Reduction Reaction Activity for Sensitive Monitoring of Organophosphorus Pesticides

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