Peroxymonosulfate Activation on Synergistically Enhanced Single-Atom Co/Co@C for Boosted Chemiluminescence of Tris(bipyridine) Ruthenium(II) Derivative

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成果类型：

期刊论文

作者：

Wu, Zhichao;Wang, Canglong;Luo, Zhen;Qin, Ying;Wang, Xiaosi;...

通讯作者：

Liuyong Hu<&wdkj&>Wenling Gu<&wdkj&>Chengzhou Zhu

作者机构：

[Luo, Zhen; Qin, Ying; Zhu, Chengzhou; Wang, Xiaosi; Gu, Wenling; Wu, Zhichao] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol, Key Lab Pesticides & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

[Wang, Canglong] Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China.

[Wang, Canglong] Adv Energy Sci & Technol Guangdong Lab, Huizhou 516000, Peoples R China.

[Wen, Jing; Hu, Liuyong] Wuhan Inst Technol, Hubei Engn Technol Res Ctr Optoelect & New Energy, Hubei Key Lab Plasma Chem & Adv Mat, Wuhan 430205, Peoples R China.

通讯机构：

[Liuyong Hu] H

[Wenling Gu; Chengzhou Zhu] K

Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, Hubei Engineering Technology Research Center of Optoelectronic and New Energy Materials, Wuhan Institute of Technology, Wuhan 430205, P. R. China<&wdkj&>Key Laboratory of Pesticides and Chemical Biology of Ministry of Education, International Joint Research Center for Intelligent Biosensing Technology and Health, College of Chemistry, Central China Normal University, Wuhan 430079, P. R. China

语种：

英文

期刊：

Analytical Chemistry

ISSN：

0003-2700

年：

2022

卷：

期：

页码：

6866-6873

DOI：

10.1021/acs.analchem.2c00881

基金类别：

National Natural Science Foundation of China [22004042, 22074049, 22104114]; Natural Science Foundation of Hubei Province [2021CFB518, 2020CFB276]; Youth Project of Hubei Provincial Department of Education [Q20211511]; State Key Laboratory of Electroanalytical Chemistry [SKLEAC202102]; Strategic Priority Research Program of Chinese Academy of Sciences [XDA21010202]; Fundamental Research Funds for the Central Universities [CCNU20QN007, CCNU20TS013]; Program of Introducing Talents of Discipline to Universities of China (111 program) [B17019]; Advanced Energy Science and Technology Guangdong Laboratory

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

Tris(bipyridine) ruthenium(II)-based luminophores have been well developed in the area of electrochemiluminescence, while their applications in chemiluminescence (CL) are rarely studied due to the poor luminous efficiency and complicated CL reaction. Herein, a novel tris(bipyridine) ruthenium(II)-based ternary CL system is proposed by introducing cobalt single atoms integrated with graphene-encapsulated cobalt nanoparticles (Co SAs/Co@C) and peroxymonosulfate (PMS) as advanced coreaction accelerator and promising coreactant, respectively. On the basis of the experimental results and density fu...

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Peroxymonosulfate Activation on Synergistically Enhanced Single-Atom Co/Co@C for Boosted Chemiluminescence of Tris(bipyridine) Ruthenium(II) Derivative

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