A Controlled Release Aptasensor Utilizing AIE-Active MOFs as High-Efficiency ECL Nanoprobe for the Sensitive Detection of Adenosine Triphosphate

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成果类型：

期刊论文

作者：

Li, Jingshuai;Xi, Mengzhen;Hu, Liuyong;Sun, Hongcheng;Zhu, Chengzhou;...

通讯作者：

Gu, WL

作者机构：

[Zhu, Chengzhou; Gu, Wenling; Li, Jingshuai; Xi, Mengzhen] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

[Hu, Liuyong] Wuhan Inst Technol, Hubei Engn Technol Res Ctr Optoelect & New Energy, Hubei Key Lab Plasma Chem & Adv Mat, Wuhan 430205, Peoples R China.

[Sun, Hongcheng] Hangzhou Normal Univ, Coll Mat Chem & Chem Engn, Key Lab Organosilicon Chem & Mat Technol, Minist Educ, Hangzhou 311121, Peoples R China.

[Gu, Wenling] Key Lab Opt Elect Sensing & Analyt Chem Life Sci, MOE, Qingdao 266042, Peoples R China.

通讯机构：

[Gu, WL ] C

Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

Key Lab Opt Elect Sensing & Analyt Chem Life Sci, MOE, Qingdao 266042, Peoples R China.

语种：

英文

期刊：

Analytical Chemistry

ISSN：

0003-2700

年：

2024

卷：

期：

页码：

2100-2106

DOI：

10.1021/acs.analchem.3c04794

基金类别：

Knowledge Innovation Program of Wuhan-Shuguang Project [22004042]; National Natural Science Foundation of China [2023AFB571]; Natural Science Foundation of Hubei Province [2023020201020441]; Knowledge Innovation Program of Wuhan-Shuguang Project [CCNU22JC006]; Fundamental Research Funds for the Central Universities [B17019]; Program of Introducing Talents of Discipline to Universities of China [M2024-1]; Open Project Program of Key Laboratory of Optic-electric Sensing and Analytical Chemistry for Life Science; MOE

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

Improving the sensitivity in electrochemiluminescence (ECL) detection systems necessitates the integration of robust ECL luminophores and efficient signal transduction. In this study, we report a novel ECL nanoprobe (Zr-MOF) that exhibits strong and stable emission by incorporating aggregation-induced emission ligands into Zr-based metal-organic frameworks (MOFs). Meanwhile, we designed a high-performance signal modulator through the implementation of a well-designed controlled release system with a self-on/off function. ZnS quantum dots (QDs) encapsulated within the cavities of aminated mesop...

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A Controlled Release Aptasensor Utilizing AIE-Active MOFs as High-Efficiency ECL Nanoprobe for the Sensitive Detection of Adenosine Triphosphate

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