EFFICIENT AMMONIA ELECTROSYNTHESIS FROM NITRATE ON STRAINED RUTHENIUM NANOCLUSTERS

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成果类型：

期刊论文

作者：

Li, Jie;Zhan, Guangming;Yang, Jianhua;Quan, Fengjiao;Mao, Chengliang;...

通讯作者：

Zhang, Lizhi;Yu, Jimmy C.

作者机构：

[Xu, Liangpang; Lei, Fengcai; Chan, Alice W. M.; Li, Lejing; Liu, Yang; Yu, Jimmy C.; Li, Jie] Chinese Univ Hong Kong, Dept Chem, Shatin, Hong Kong, Peoples R China.

[Quan, Fengjiao; Zhang, Lizhi; Shi, Yanbiao; Mao, Chengliang; Zhan, Guangming] Cent China Normal Univ, Coll Chem, Inst Environm & Appl Chem, Minist Educ,Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China.

[Wang, Jianfang; Yang, Jianhua] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China.

[Wong, Po Keung; Wang, Bo] Chinese Univ Hong Kong, Sch Life Sci, Shatin, Hong Kong, Peoples R China.

[Du, Yi; Dou, Shi-Xue] Univ Wollongong, AIIM, ISEM, Wollongong, NSW 2500, Australia.

通讯机构：

[Zhang, Lizhi; Yu, Jimmy C.] C

Cent China Normal Univ, Coll Chem, Inst Environm & Appl Chem, Minist Educ,Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China.

Chinese Univ Hong Kong, Dept Chem, Shatin, Hong Kong, Peoples R China.

语种：

英文

期刊：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

ISSN：

0002-7863

年：

2020

卷：

142

期：

页码：

7036-7046

DOI：

10.1021/jacs.0c00418

基金类别：

This work was financially supported by the Research Grants Council of the Hong Kong Special Administrative Region (project no. 14304019), the Natural Science Funds for Distinguished Young Scholars (grant no. 21425728), the National Science Foundation of China (grant no. 51472100), the 111 Project (grant no. B17019), and the Australian Research Council (DP160102627, DP170101467, and FT180100585). This work has benefited from the National Synchrotron Radiation Laboratory in Beijing and Shanghai for characterization. We thank the National Supercomputer Center in Jinan for providing high-performance computing.

机构署名：

本校为通讯机构

院系归属：

化学学院

摘要：

The limitations of the Haber-Bosch reaction, particularly high-temperature operation, have ignited new interests in low-temperature ammonia-synthesis scenarios. Ambient N-2 electroreduction is a compelling alternative but is impeded by a low ammonia production rate (mostly

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