Manipulation of aurophilicity in constructed clusters of gold(I) complexes with boosted luminescence and smart responsiveness

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成果类型：

期刊论文

作者：

Peng, Zhen;Zhang, Jianyu;Feng, Na;Zhang, Jing;Liu, Sheng Hua

通讯作者：

Liu, SH;Zhang, J

作者机构：

[Peng, Zhen; Liu, Sheng Hua; Liu, SH] Cent China Normal Univ, Coll Chem, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

[Zhang, Jing; Feng, Na; Zhang, J] Southern Med Univ, Nanfang Hosp, Dept Lab Med, Guangzhou 510515, Peoples R China.

[Zhang, Jianyu] Hong Kong Univ Sci & Technol, Hong Kong Branch, Chinese Natl Engn Res Ctr Tissue Restorat & Recons, Dept Chem,Kowloon, Clear Water Bay, Hong Kong 999077, Peoples R China.

[Zhang, Jianyu] Hong Kong Univ Sci & Technol, Inst Adv Study, Kowloon, Clear Water Bay, Hong Kong 999077, Peoples R China.

通讯机构：

[Liu, SH ] C

[Zhang, J ] S

Cent China Normal Univ, Coll Chem, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

Southern Med Univ, Nanfang Hosp, Dept Lab Med, Guangzhou 510515, Peoples R China.

语种：

英文

关键词：

Aggregation-induced emission;Aurophilic interaction;Gold complex;Mechanoluminochromism

期刊：

SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY

ISSN：

1386-1425

年：

2024

卷：

311

页码：

123979

DOI：

10.1016/j.saa.2024.123979

基金类别：

National Natural Science Foundation of China [22175069, 22205096]; The 111 Project [B17019]; Outstanding Youths Development Scheme of Nanfang Hospital, Southern Medical University [2021J002]; GuangDong Basic and Applied Basic Research Foundation [2021A1515110373, 2023A1515011924]

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

High-performance luminescent gold(I) complexes have attracted considerable attention due to their potential applications in various fields, but their construction is a significantly challenging task. Herein, we designed and synthesized a series of novel dinuclear gold(I) complexes 1-4 based on 1,2-bis(diphenylphosphino)benzene and 1,4-bis(diphenylphosphino)benzene frameworks, where para-substitutions of benzene ring were employed for comparison and bulky t-butyl groups were introduced into carbazole ligands to assist flexibly regulating the aurophilicity. Among them, the structure of complex 1...

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Manipulation of aurophilicity in constructed clusters of gold(I) complexes with boosted luminescence and smart responsiveness

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