期刊论文

Zhang, Lizhi

英文

Environmental Science & Technology

0013-936X

2017

51

10

5685-5694

10.1021/acs.est.7b00040

National Natural Science Funds for Distinguished Young ScholarsNational Natural Science Foundation of China (NSFC)National Science Fund for Distinguished Young Scholars [21425728]; National Basic Research Program of China (973 Program)National Basic Research Program of China [2013CB632402]; National Key Research and Development Program of China [2016YFA0203002]; National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51472100]; 111 ProjectMinistry of Education, China - 111 Project [B17019]; Excellent Doctorial Dissertation Cultivation Grant from Central China Normal University [2015YBZD018, 2016YBZZ034]; CAS Interdisciplinary Innovation Team of the Chinese Academy of Sciences

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Understanding the chemistry of hydrogen peroxide (H2O2) decomposition and hydroxyl radical (•OH) transformation on the surface molecular level is a great challenge for the application of heterogeneous Fenton system in the fields of chemistry, environmental, and life science. We report in this study a conceptual oxygen vacancy associated surface Fenton system without any metal ions leaching, exhibiting unprecedented surface chemistry based on the oxygen vacancy of electron-donor nature for heterolytic H2O2 dissociation. By controlling the delic...