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Vacancy-Rich and Porous NiFe-Layered Double Hydroxide Ultrathin Nanosheets for Efficient Photocatalytic NO Oxidation and Storage

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成果类型:
期刊论文
作者:
Li, Hao;Zhu, Huijun;Shi, Yanbiao;Shang, Huan;Zhang, Lizhi;...
通讯作者:
Wang, Jing
作者机构:
[Li, Hao; Wang, Jing] Inst Environm Engn, CH-8093 Zurich, Switzerland.
[Li, Hao; Wang, Jing] Empa, Swiss Fed Labs Mat Sci & Technol, Lab Adv Analyt Technol, CH-8600 Dubendorf, Switzerland.
[Zhu, Huijun] Linkoping Univ, S-58183 Linkoping, Sweden.
[Zhang, Lizhi; Shi, Yanbiao] Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, Shanghai 200240, Peoples R China.
[Zhang, Lizhi; Shang, Huan] Cent China Normal Univ, Coll Chem, Inst Appl & Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
通讯机构:
[Wang, Jing] I
[Wang, Jing] S
Inst Environm Engn, CH-8093 Zurich, Switzerland.
Swiss Fed Labs Mat Sci & Technol, Empa, Lab Adv Analyt Technol, CH-8600 Dubendorf, Switzerland.
语种:
英文
关键词:
photocatalysis;NO removal;layered double hydroxide;environmental control;nitrate storage
期刊:
Environmental Science & Technology
ISSN:
0013-936X
年:
2022
卷:
56
期:
3
页码:
1771-1779
基金类别:
This work was supported by ETH Zürich and Center for Filtration Research (CFR) at the University of Minnesota.
机构署名:
本校为其他机构
院系归属:
化学学院
摘要:
An appealing strategy in the direction of circular chemistry and sustainable nitrogen exploitation is to efficiently convert NOx pollutants into low-toxic products and simultaneously provide crop plants with metabolic nitrogen. This study demonstrates that such a scenario can be realized by a defect- and morphology-coengineered Ni-Fe-layered double hydroxide (NiFe-LDH) comprising ultrathin nanosheets. Rich oxygen vacancies are introduced onto the NiFe-LDH surface, which facilitate charge carrier transfer and enable photocatalytic O2 activation ...

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