[Zhang, Lizhi; Fang, Chuyang; Zhan, Guangming] Cent China Normal Univ, Coll Chem, Inst Appl & Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
通讯机构:
[Prof. Lizhi Zhang] S
School of Environmental Science and Engineering, Shanghai Jiao Tong University, Shanghai, 200240 P. R. China<&wdkj&>Key Laboratory of Pesticide & Chemical Biology of Ministry of Education Institute of Applied & Environmental Chemistry College of Chemistry, Central China Normal University, Wuhan, 430079 P. R. China
National Natural Science Foundation of China [22102100, 21936003]; Natural Science Foundation of Shanghai [22ZR1431700]; National Key Research and Development Program of China [2021YFA1201701, 2018YFC1800801]
机构署名:
本校为其他机构
院系归属:
化学学院
摘要:
Fabricating single-atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab-to-fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand-free isolated Ru atoms on the amorphous layer of monolithic Ti support by regulating the electronic metal-support interactions. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution activity, three orders of magnitude higher ma...