期刊论文

Cheng, Ying;Xiao, Wen-Jing

英文

Chemical Communications

1359-7345

2020

56

77

11508-11511

10.1039/d0cc05167e

National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21901080, 91956201, 21820102003, 21772053]; Program of Introducing Talents of Discipline to Universities of China (111 Program) [B17019]; Natural Science Foundation of Hubei ProvinceNatural Science Foundation of Hubei Province [2017AHB047]; International Joint Research Centre for Intelligent Biosensing Technology and Health

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An unprecedented triple catalytic, general ring-opening cyanation reaction of cyclopropyl ketones for the construction of γ-cyanoketones is described. The key is to merge photoredox catalysis with Lewis acid catalysis and copper catalysis to enable the selective cleavage of the carbon-carbon bonds and the selective coupling of the generated radical and cyan...