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Ascorbic acid/Fe@Fe2O3: A highly efficient combined Fenton reagent to remove organic contaminants

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成果类型:
期刊论文
作者:
Hou, Xiaojing;Huang, Xiaopeng;Ai, Zhihui*;Zhao, Jincai;Zhang, Lizhi*
通讯作者:
Ai, Zhihui;Zhang, Lizhi
作者机构:
[Zhang, Lizhi; Hou, Xiaojing; Huang, Xiaopeng; Zhao, Jincai; Ai, ZH; Zhang, LZ; Ai, Zhihui] Cent China Normal Univ, Inst Environm Chem, Coll Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
通讯机构:
[Ai, ZH; Zhang, LZ] C
Cent China Normal Univ, Inst Environm Chem, Coll Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
语种:
英文
关键词:
Alachlor;Ascorbic acid;Degradation;Fe@Fe(2)O(3) core-shell nanowires;Fenton reaction
期刊:
Journal of Hazardous Materials
ISSN:
0304-3894
年:
2016
卷:
310
页码:
170-178
基金类别:
National Natural Science Funds for Distinguished Young ScholarsNational Natural Science Foundation of China (NSFC)National Science Fund for Distinguished Young Scholars [21425728]; National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21173093, 21177048, 21477044]; Natural Science Foundation of Hubei ProvinceNatural Science Foundation of Hubei Province [2013CFA114]; Self-Determined Research Funds of CCNU from the Colleges' Basic Research and Operation of MOE [CCNU14Z01001, CCNU14KFY002]
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
In this study, we demonstrate that the combination of ascorbic acid and Fe@Fe2O3core-shell nanowires (AA/Fe@Fe2O3) offers a highly efficient Fenton reagent. This combined Fenton reagent exhibited extremely high activity on the decomposition of H2O2to produce OH for the degradation of various organic contaminants, including rhodamine B, methylene blue, alachlor, atrazine, siduron, lincomycin, and chloroamphenicol. The contaminant degradation constants in the AA/Fe@Fe2O3/H2O2Fenton systems were 38-53 times higher than those in the conventional homogeneous Fenton system (Fe(II)/H2O2) at pH 3.8. M...

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