Selective Three-Component 1,2-Aminoalkoxylation of 1-Aryl-1,3-dienes by Dual Photoredox and Copper Catalysis

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作者信息关键词期刊信息基础信息归属信息摘要

成果类型：

期刊论文

作者：

Wu, Ya-Li;Jiang, Min;Rao, Li;Cheng, Ying;Xiao, Wen-Jing;...

通讯作者：

Jia-Rong Chen

作者机构：

[Cheng, Ying; Rao, Li; Xiao, Wen-Jing; Chen, Jia-Rong; Wu, Ya-Li] Cent China Normal Univ, Coll Chem, Minist Educ, CCNU uOttawa Joint Res Ctr,Key Lab Pesticides & Ch, Wuhan 430079, Peoples R China.

[Jiang, Min] Hangzhou Normal Univ, Coll Mat Chem & Chem Engn, Hangzhou 310036, Peoples R China.

[Chen, Jia-Rong] Henan Normal Univ, Sch Chem & Chem Engn, Xinxiang 453007, Peoples R China.

通讯机构：

[Jia-Rong Chen] C

CCNU-uOttawa Joint Research Centre, Key Laboratory of Pesticides & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, Wuhan 430079, P. R. China<&wdkj&>School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, P. R. China

语种：

英文

期刊：

Organic Letters

ISSN：

1523-7060

年：

2022

卷：

期：

页码：

7470-7475

DOI：

10.1021/acs.orglett.2c03124

基金类别：

National Natural Science Foundation of China [21971081, 22171099, 21820102003, 21901080, 91956201]; School of Chemistry and Chemical Engineering, Henan Normal University [2021YB02]; Program of Introducing Talents of Discipline to Universities of China(111 Program) [B17019]

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

A three-component 1,2-aminooxygenation reaction of 1,3-dienes by dual photoredox and copper catalysis is described. This protocol uses N-aminopyridinium salts as N-centered radical precursors and nucleophilic alcohols as oxygen sources, providing modular and practical access to 1,2-aminoalkoxylation products with good yields and regioselectivity. Preliminary mechanistic studies support the radical property of the reaction and th...

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Selective Three-Component 1,2-Aminoalkoxylation of 1-Aryl-1,3-dienes by Dual Photoredox and Copper Catalysis

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