Bottom-Up Construction of Ni(II)-Incorporated Covalent Organic Framework for Metallaphotoredox Catalysis

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成果类型：

期刊论文

作者：

Hu, Hai-Chao;Wang, Zhi-Peng;Liang, Lin;Du, Xin-Yu;Li, Ting;...

通讯作者：

Liu, Qiang;Wang, W;Lu, Liang-Qiu;Xiao, WJ

作者机构：

[Feng, Jie; Wang, Wei; Liu, Qiang; Xiao, Tian-Tian; Ding, San-Yuan; Hu, Hai-Chao; Jin, Ze-Ming; Li, Ting; Du, Xin-Yu; Wang, Zhi-Peng; Liang, Lin] Lanzhou Univ, Coll Chem & Chem Engn, State Key Lab Appl Organ Chem, Lanzhou 730000, Gansu, Peoples R China.

[Lu, Liang-Qiu; Xiao, Wen-Jing; Lu, LQ] Cent China Normal Univ, Coll Chem, Engn Res Ctr Photoenergy Utilizat Pollut Control &, Minist Educ, 152 Luoyu Rd, Wuhan 430079, Hubei, Peoples R China.

通讯机构：

[Wang, W ; Liu, Q] L

[Lu, LQ; Xiao, WJ ] C

Lanzhou Univ, Coll Chem & Chem Engn, State Key Lab Appl Organ Chem, Lanzhou 730000, Gansu, Peoples R China.

Cent China Normal Univ, Coll Chem, Engn Res Ctr Photoenergy Utilizat Pollut Control &, Minist Educ, 152 Luoyu Rd, Wuhan 430079, Hubei, Peoples R China.

语种：

英文

关键词：

covalent organic framework;metallaphotoredox catalysis;bottom-up strategy;cross-coupling reactions

期刊：

CHEMISTRY-A EUROPEAN JOURNAL

ISSN：

0947-6539

年：

2024

卷：

期：

页码：

e202303476-

DOI：

10.1002/chem.202303476

基金类别：

National Key R&D Program of China; National Natural Science Foundation of China [92056202]; Scientific Research Program of Gansu Provincial Department of Education [202ljyjbgs-04]; [2022YFA1503300]

机构署名：

本校为通讯机构

院系归属：

化学学院

摘要：

We developed a facile bottom‐up strategy to synthesize Ni(II)‐incorporated covalent organic framework (LZU‐713@Ni) as heterogeneous all‐in‐one metallaphotoredox catalyst. LZU‐713@Ni showed excellent activity and recyclability in photoredox/nickel‐catalyzed C−O, C−S, and C−P cross‐coupling reactions. The superiority of bottom‐up strategy was exemplified by the increased activity of LZU‐713@Ni compared to both the dual catalyst system and LZU‐713/Ni prepared via post‐synthetic modification. Abstract The construction of an all‐in‐...

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Bottom-Up Construction of Ni(II)-Incorporated Covalent Organic Framework for Metallaphotoredox Catalysis

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