Mass spectrometric monitoring of ligand-bridged hot electron transfer and anaerobic oxidization on auto renewable droplet-based plasmonic nanoreactors under visible light illumination

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成果类型：

期刊论文

作者：

Shen, Baojie;Chen, Disong;Li, Rui;Qi, Yinghua;Gao, Anji;...

通讯作者：

Zhong, HY

作者机构：

[Shen, Baojie; Qi, Yinghua; Chen, Disong; Li, Rui] Cent China Normal Univ, Coll Chem, Lab Mass Spectrometry, Wuhan 430079, Hubei, Peoples R China.

[Zhong, Hongying; Zhong, HY] Guangxi Univ, Coll Life Sci & Technol, Ctr Instrumental Anal, Nanning 530004, Guangxi, Peoples R China.

[Gao, Anji] Chinese Acad Sci, Innovat Acad Precis Measurement Sci & Technol, Wuhan 430071, Peoples R China.

[Gao, Anji] Univ Chinese Acad Sci, Beijing 100049, Peoples R China.

通讯机构：

[Zhong, HY ] G

Guangxi Univ, Coll Life Sci & Technol, Ctr Instrumental Anal, Nanning 530004, Guangxi, Peoples R China.

语种：

英文

关键词：

Anaerobic oxidization;Hot electrons;Ligand-bridged electron transfer;Mass spectrometry;Plasmonic nanoreactors

期刊：

Analytica Chimica Acta

ISSN：

0003-2670

年：

2023

卷：

1283

页码：

341965

DOI：

10.1016/j.aca.2023.341965

基金类别：

National Natural Science Foundation of China [NSFC 21834002, 81761128005]; Central China Normal University; Guangxi University

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

The light induced hot-electron on plasmonic nanostructures has been recognized as a breakthrough discovery for photovoltaic and photocatalytic applications. With mass spectrometry, we demonstrate the dynamics of hot electron transfers of anaerobic oxidization reactions on Au decorated TiO2 plasmonic nanoparticles, which were coated on the inner surface of a flask. Those nanoparticles were covered by continuously renewed liquid droplets of solvent and reactants that were transported through a Venturi jet mixer with auto-spray. In addition to intensive mass transfer in such droplet-based nanorea...

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Mass spectrometric monitoring of ligand-bridged hot electron transfer and anaerobic oxidization on auto renewable droplet-based plasmonic nanoreactors under visible light illumination

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