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[4+3] Cycloaddition of in situ generated azoalkenes with C,N-cyclic azomethine imines: efficient synthesis of tetrazepine derivatives

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成果类型:
期刊论文、会议论文
作者:
Hu, Xiao-Qiang;Chen, Jia-Rong*;Gao, Shuang;Feng, Bin;Lu, Liang-Qiu;...
通讯作者:
Chen, Jia-Rong
作者机构:
[Feng, Bin; Lu, Liang-Qiu; Xiao, Wen-Jing; Chen, Jia-Rong; Gao, Shuang; Hu, Xiao-Qiang] Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Hubei, Peoples R China.
[Chen, Jia-Rong] Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, 152 Luoyu Rd, Wuhan 430079, Hubei, Peoples R China.
通讯机构:
[Chen, Jia-Rong] C
Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, 152 Luoyu Rd, Wuhan 430079, Hubei, Peoples R China.
语种:
英文
关键词:
[4+3] cycloaddition;azomethine imines;1,2-diaza-1,3-dienes;tetrazepine
期刊:
Chemical Communications
ISSN:
1359-7345
年:
2013
卷:
49
期:
72
页码:
7905-7907
会议名称:
中国化学会第八届有机化学学术会议暨首届重庆有机化学国际研讨会
会议时间:
2013-10-17
会议地点:
中国重庆
基金类别:
National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21002036, 21272087, 21202053, 21232003]; National Basic Research Program of ChinaNational Basic Research Program of China [2011CB808603]
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
An unprecedented [4+3] cycloaddition of in situ generated azoalkenes with C,N-cyclic azomethine imines has been developed without the use of any catalyst, providing an efficient and mild approach to synthesise highly functionalized 1,2,4,5-tetrazepine derivatives in high yields (76-92%)....

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