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Recent advances of ammonia synthesis under ambient conditions over metal-organic framework based electrocatalysts

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成果类型:
期刊论文
作者:
Yu, Yu;Li, Yuan;Fang, Yu;Wen, Lili;Tu, Binbin;...
通讯作者:
Huang, Y
作者机构:
[Li, Yuan; Fang, Yu; Yu, Yu] Anhui Univ, Sch Chem & Chem Engn, Hefei 230601, Peoples R China.
[Tu, Binbin; Huang, Yi; Wen, Lili] Cent China Normal Univ, Coll Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.
通讯机构:
[Huang, Y ] C
Cent China Normal Univ, Coll Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.
语种:
英文
关键词:
Ammonia electrosynthesis;Electrocatalytic reduction reactions;Metal-organic frameworks (MOFs);MOFs derivatives
期刊:
Applied Catalysis B: Environmental
ISSN:
0926-3373
年:
2024
卷:
340
页码:
123161
基金类别:
National Natural Science Foundation of China [U21A20286, 22206054]; Natural Science Foundation of Hubei [ZRMS2021000800]; Fundamental Research Funds for the Central China Normal University (CCNU); Anhui University [S020318008/015]
机构署名:
本校为通讯机构
院系归属:
化学学院
摘要:
Ammonia (NH3) is an essential chemical and a promising fuel, but its industrially produced process is carbon-intensive and highly energy-consuming. Developing a green and sustainable NH3 synthesis route is extremely urgent. Electrochemical ammonia synthesis (EAS) powered by renewable electricity energy under ambient conditions is fascinating, while exploring the efficient electrocatalysts and suitable nitrogen source is critical. Due to the unique characteristics of adjustable porosity and component, large specific surface area and diverse structure, metal-organic frameworks (MOFs) and their v...

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