Deaminative (Carbonylative) Alkyl‐Heck‐type Reactions Enabled by Photocatalytic C−N Bond Activation

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期刊论文

作者：

Xuan Jiang;Mao-Mao Zhang;Wei Xiong;Prof. Dr. Liang-Qiu Lu;Prof. Dr. Wen-Jing Xiao;...

通讯作者：

Prof. Dr. Liang-Qiu Lu<&wdkj&>Prof. Dr. Wen-Jing Xiao<&wdkj&>Prof. Dr. Liang-Qiu Lu Prof. Dr. Liang-Qiu Lu Prof. Dr. Liang-Qiu Lu<&wdkj&>Prof. Dr. Wen-Jing Xiao Prof. Dr. Wen-Jing Xiao Prof. Dr. Wen-Jing Xiao

作者机构：

[Xuan Jiang; Mao-Mao Zhang; Wei Xiong; Prof. Dr. Liang-Qiu Lu; Xuan Jiang Xuan Jiang Xuan Jiang; Mao-Mao Zhang Mao-Mao Zhang Mao-Mao Zhang; Wei Xiong Wei Xiong Wei Xiong; Prof. Dr. Liang-Qiu Lu Prof. Dr. Liang-Qiu Lu Prof. Dr. Liang-Qiu Lu] Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei, 430079 China

State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai, 200032 China

[Prof. Dr. Wen-Jing Xiao; Prof. Dr. Wen-Jing Xiao Prof. Dr. Wen-Jing Xiao Prof. Dr. Wen-Jing Xiao] Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei, 430079 China<&wdkj&>State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai, 200032 China

通讯机构：

[Prof. Dr. Liang-Qiu Lu; Prof. Dr. Wen-Jing Xiao; Prof. Dr. Liang-Qiu Lu Prof. Dr. Liang-Qiu Lu Prof. Dr. Liang-Qiu Lu; Prof. Dr. Wen-Jing Xiao Prof. Dr. Wen-Jing Xiao Prof. Dr. Wen-Jing Xiao] K

Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei, 430079 China<&wdkj&>Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei, 430079 China<&wdkj&>State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai, 200032 China

语种：

英文

关键词：

Amine;Carbonylierende Reaktionen;Desaminierende Umsetzungen;Heck-Reaktion;Photokatalyse

期刊：

Angewandte Chemie

ISSN：

0044-8249

年：

2019

卷：

131

期：

页码：

2424-2428

DOI：

10.1002/ange.201813689

基金类别：

National Natural Science Foundation of China#&#&#21822103, 21820102003, 21772052, 21772053, 21572074 and 21472057

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

AbstractThe palladium‐catalyzed Heck reaction is a well‐known, Nobel Prize winning transformation for producing alkenes. Unlike the alkenyl and aryl variants of the Heck reaction, the alkyl‐Heck reaction is still underdeveloped owing to the competitive side reactions of alkyl–palladium species. Herein, we describe the development of a deaminative alkyl‐Heck‐type reaction that proceeds through C−N bond activation by visible‐light photoredox catalysis. A variety of aliphatic primary amines were found to be efficient starting materials for...

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Deaminative (Carbonylative) Alkyl‐Heck‐type Reactions Enabled by Photocatalytic C−N Bond Activation

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