Small-Molecule Probe-Induced In Situ-Sensitized Photoelectrochemical Biosensor for Monitoring & alpha;-Glucosidase Activity

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成果类型：

期刊论文

作者：

Qin, Ying;Zhang, Jingyi;Tan, Rong;Wu, Zhichao;Liu, Mingwang;...

通讯作者：

Gu, WL;Hu, LY

作者机构：

[Qin, Ying; Zhu, Chengzhou; Liu, Mingwang; Li, Jinli; Xu, Miao; Tan, Rong; Gu, Wenling; Wu, Zhichao; Zhang, Jingyi] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

[Hu, Liuyong] Wuhan Inst Technol, Hubei Engn Technol Res Ctr Optoelect & New Energy, Hubei Key Lab Plasma Chem & Adv Mat, Wuhan 430205, Peoples R China.

[Gu, Wenling] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

通讯机构：

[Hu, LY ; Gu, WL ]

Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol &, Natl Key Lab Green Pesticide, Wuhan 430079, Peoples R China.

Wuhan Inst Technol, Hubei Engn Technol Res Ctr Optoelect & New Energy, Hubei Key Lab Plasma Chem & Adv Mat, Wuhan 430205, Peoples R China.

语种：

英文

关键词：

carbon nitride;in situ sensitization;photoelectrochemical biosensor;small-molecule probe;α-glucosidase

期刊：

ACS SENSORS

ISSN：

2379-3694

年：

2023

卷：

期：

页码：

3257–3263

DOI：

10.1021/acssensors.3c01269

基金类别：

National Natural Science Foundation of China [22104114]; Natural Science Foundation of Hubei Province [2021CFB518]; Fundamental Research Funds for the Central Universities [CCNU22JC006]; Program of Introducing Talents of Discipline to Universities of China (111 program) [B17019]

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

Semiconductor-based photoelectrochemical (PEC) biosensors have garnered significant attention in the field of disease diagnosis and treatment. However, the recognition units of these biosensors are mainly limited to bioactive macromolecules, which hinder the photoelectric response due to their insulating characteristics. In this study, we develop an in situ-sensitized strategy that utilizes a small-molecule probe at the interface of the photoelectrode to accurately detect α-glucosidase (α-Glu) activity. Silane, a prototype small-molecule prob...

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Small-Molecule Probe-Induced In Situ-Sensitized Photoelectrochemical Biosensor for Monitoring & alpha;-Glucosidase Activity

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