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Highly efficient electrochemical conversion of CO2 and NaCl to CO and NaClO

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成果类型:
期刊论文
作者:
Quan, Fengjiao;Zhan, Guangming;Shang, Huan;Huang, Yahui;Jia, Falong*;...
通讯作者:
Jia, Falong;Ai, Zhihui
作者机构:
[Quan, Fengjiao; Zhang, Lizhi; Huang, Yahui; Shang, Huan; Jia, Falong; Ai, ZH; Zhan, Guangming; Ai, Zhihui] Cent China Normal Univ, Inst Appl & Environm Chem, Coll Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Hubei, Peoples R China.
通讯机构:
[Jia, FL; Ai, ZH] C
Cent China Normal Univ, Inst Appl & Environm Chem, Coll Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Hubei, Peoples R China.
语种:
英文
期刊:
Green Chemistry
ISSN:
1463-9262
年:
2019
卷:
21
期:
12
页码:
3256-3262
基金类别:
National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21777050, 21872061, 21876058]; National Key Research and Development Program of China [2016YFA0203002]; National Natural Science Funds for Distinguished Young ScholarsNational Natural Science Foundation of China (NSFC)National Science Fund for Distinguished Young Scholars [21425728]
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
A robust electrocatalyst based on single iron atoms was developed for CO2 reduction with a high faradaic efficiency over 99.6%. The cathodic CO2 reduction was then coupled with anodic production of hypochlorite, and high energy efficiency (82%) with nearly 100% atom economy could be achieved in this model electrolysis system....

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