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Facile fabrication of rGO/PPy/nZVI catalytic microreactor for ultrafast removal of p-nitrophenol from water

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成果类型:
期刊论文
作者:
Chen, Yanyan;Zhang, Manlin;Chen, Tiantian;Zhang, Ganbing;Xu, Hui*;...
通讯作者:
Xu, Hui;Sun, HW
作者机构:
[Zhang, Manlin; Sun, Hongwei; Xu, Hui; Chen, Tiantian; Chen, Yanyan] Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China.
[Zhang, Lizhi] Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, Shanghai 200240, Peoples R China.
[Zhang, Ganbing] Hubei Univ, Coll Chem & Chem Engn, Wuhan 430062, Peoples R China.
通讯机构:
[Xu, H; Sun, HW ] C
Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China.
语种:
英文
关键词:
Zerovalent iron;Graphene;Microreactor;Fenton-like reaction;P-nitrophenol
期刊:
Applied Catalysis B: Environmental
ISSN:
0926-3373
年:
2023
卷:
324
页码:
122270
基金类别:
CRediT authorship contribution statement Yanyan Chen: Investigation, Visualization, Writing − original draft. Manlin Zhang: Investigation. Tiantian Chen: Validation. Ganbing Zhang: Investigation. Hui Xu: Methodology, Supervision, Writing − review & editing, acquisition. Hongwei Sun: Methodology, Writing − review & editing, acquisition. Lizhi Zhang: Writing − review & editing, Supervision.
机构署名:
本校为第一且通讯机构
院系归属:
化学学院
摘要:
The application of powdered nanoscale zero-valent iron (nZVI) in conventional reactors for water treatment is limited by insufficient mass-transfer and difficult post-separation of catalysts. Herein, a novel microreactor was constructed by anchoring nZVI on the reduced graphene oxide/polypyrrole nanocomposite (rGO/PPy) substrate within the microchannel of a stainless-steel tube through two-step electrodeposition, which catalyzed the Fenton-like reaction to remove > 99% p-nitrophenol (PNP) within 50 s, outperforming traditional batch reactors. T...

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