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Facet-level mechanistic insights into general homogeneous carbon doping for enhanced solar-to-hydrogen conversion

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成果类型:
期刊论文
作者:
Li, Jie*;Zhao, Kun;Yu, Ying;Zhang, Lizhi
通讯作者:
Li, Jie
作者机构:
[Zhang, Lizhi; Li, Jie; Zhao, Kun] Cent China Normal Univ, Coll Chem, Inst Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
[Li, Jie; Yu, Ying] Cent China Normal Univ, Coll Phys Sci & Technol, Inst Nanosci & Nanotechnol, Wuhan 430079, Peoples R China.
通讯机构:
[Li, Jie] C
Cent China Normal Univ, Coll Chem, Inst Environm Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.
语种:
英文
关键词:
BiOCl;carbon doping;facet exposure;photocatalysis;solar-to-hydrogen conversion
期刊:
Advanced Functional Materials
ISSN:
1616-301X
年:
2015
卷:
25
期:
14
页码:
2189-2201
基金类别:
National Natural Science Funds for Distinguished Young ScholarsNational Natural Science Foundation of China (NSFC)National Science Fund for Distinguished Young Scholars [21425728]; National Basic Research Program of China (973 Program)National Basic Research Program of China [2013CB632402]; National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21177048, 21377044, 51472100]; Key Project of Natural Science Foundation of Hubei ProvinceNatural Science Foundation of Hubei Province [2013CFA114]; Self-Determined Research Funds of CCNU from the Colleges' Basic Research and Operation of MOE [CCNU14Z01001]
机构署名:
本校为第一且通讯机构
院系归属:
物理科学与技术学院
化学学院
摘要:
Homogeneous doping can boost solar-to-hydrogen conversion and therefore attracts great attention. Although a great deal of effort has been made to explore the doping-photoreactivity relationship, the doping mechanisms, especially from the perspective of crystal facets, are seldom explored. In this study, a general homogeneous carbon doping strategy is established and then serves as the doping model for a mechanistic investigation, as encouraged by its versatility in enabling homogeneous incorporation of carbon and improving solar-to-hydrogen co...

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