The effect of water on the heterogeneous reactions of SO2 and NH3 on the surfaces of α-Fe2O3 and γ-Al2O3

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成果类型：

期刊论文

作者：

Yang, Weiwei;Ma, Qingxin*;Liu, Yongchun;Ma, Jinzhu;Chu, Biwu;...

通讯作者：

Ma, Qingxin

作者机构：

[Ma, Jinzhu; He, Hong; Yang, Weiwei; Liu, Yongchun; Chu, Biwu; Ma, Qingxin] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100085, Peoples R China.

[Ma, Jinzhu; He, Hong; Yang, Weiwei; Chu, Biwu; Ma, Qingxin] Univ Chinese Acad Sci, Coll Resources & Environm, Beijing 100049, Peoples R China.

[Ma, Jinzhu; He, Hong; Chu, Biwu; Ma, Qingxin] Chinese Acad Sci, Ctr Excellence Urban Atmospher Environm, Inst Urban Environm, Xiamen 361021, Fujian, Peoples R China.

[Yang, Weiwei] Cent China Normal Univ, Coll Chem, Inst Environm & Appl Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Hubei, Peoples R China.

通讯机构：

[Ma, Qingxin] C

[Ma, Qingxin] U

Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100085, Peoples R China.

Univ Chinese Acad Sci, Coll Resources & Environm, Beijing 100049, Peoples R China.

Chinese Acad Sci, Ctr Excellence Urban Atmospher Environm, Inst Urban Environm, Xiamen 361021, Fujian, Peoples R China.

语种：

英文

期刊：

Environmental Science: Nano

ISSN：

2051-8153

年：

2019

卷：

期：

页码：

2749-2758

DOI：

10.1039/c9en00574a

基金类别：

Ministry of Science and Technology of ChinaMinistry of Science and Technology, China [2016YFC0202700]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21876185, 21407158, 91744205]; Youth Innovation Promotion Association, CAS [2018055]; Young Talent Project of the Center for Excellence in Regional Atmospheric Environment, CAS [CERAE201801]

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本校为其他机构

院系归属：

化学学院

摘要：

In this study, a wall-coated flow tube reactor, in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) and ion chromatography (IC) were used to investigate the effect of water on the heterogeneous reactions of SO2 and NH3 on the surfaces of α-Fe2O3 and γ-Al2O3. Flow tube results show that water exhibited little effect on the initial uptake coefficients (γBET) of SO2 but the addition of NH3 increased the γBET at various relative humidity (RH) values on both α-Fe2O3 and γ-Al2O3. The γBET of SO2 in the presence of NH3 ...

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The effect of water on the heterogeneous reactions of SO2 and NH3 on the surfaces of α-Fe2O3 and γ-Al2O3

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