Novel amino-functionalized Ni(II)-based MOFs for efficiently photocatalytic reduction of CO2 to CO with superior selectivity under visible-light illumination

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成果类型：

期刊论文

作者：

Yang, Heng;Lai, Chunlin;Wu, Mengling;Wang, Shaodan;Xia, Yang;...

通讯作者：

Wen, Lili(wenlili@mail.ccnu.edu.cn)

作者机构：

[Lai, Chunlin; Yang, Heng; Pan, Fangfang; Wu, Mengling; Wen, Lili; Wang, Shaodan] Cent China Normal Univ, Coll Chem, Key Lab Pesticide & Chem Biol, Minist Educ, Wuhan 430079, Peoples R China.

[Xia, Yang] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China.

[Lv, Kangle] South Cent Minzu Univ, Key Lab Catalysis & Energy Mat Chem, Minist Educ, Wuhan 430074, Peoples R China.

[Wen, Lili] Chinese Acad Sci, Fujian Inst Res Struct Matter, State Key Lab Struct Chem, Fuzhou 350002, Peoples R China.

通讯机构：

[Lili Wen] K

Key Laboratory of Pesticide & Chemical Biology of Ministry of Education, College of Chemistry, Central China Normal University, Wuhan 430079, PR China<&wdkj&>State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, PR China

语种：

英文

关键词：

CO2RR;High AQE;MOFs;Open Ni(II) sites;Superior selectivity

期刊：

Chemical Engineering Journal

ISSN：

1385-8947

年：

2023

卷：

455

页码：

140425

DOI：

10.1016/j.cej.2022.140425

基金类别：

This work was financially supported by the National Nature Science Foundation of China (Nos. 22171097 , 21771072 and 22108211 ), and the Fundamental Research Funds for the Central Universities (Grant No. CCNU22QN008 and WUT: 2021IVA019B ), as well as the fund of the Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education & Hubei Key Laboratory of Catalysis and Materials Science, CHCL 21001.

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

Metal-organic frameworks (MOFs) have aroused ever-growing scientific interest for photocatalytic CO2 reduction reaction (CO2RR). Delicate design and synthesis of MOFs with open metal sites (OMSs) is the key to activate CO2 and even stabilize the reaction intermediates of CO2RR, further determine the superior selectivity. Herein, two amino-functionalized MOFs (Ni-Bpyb and Ni-Bipy) with open Ni(II) sites were constructed from 2′-amino-5′-(4-carboxyphenyl)-[1,1′:3′,1″-terphenyl]-4,4″-dicarboxylic acid (NH2-BTBH3) and different lengths of lin...

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Novel amino-functionalized Ni(II)-based MOFs for efficiently photocatalytic reduction of CO2 to CO with superior selectivity under visible-light illumination

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