Copper-Catalyzed Three-Component Photo-ATRA-Type Reaction for Asymmetric Intermolecular C-O Coupling

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成果类型：

期刊论文

作者：

Wang, Peng-Zi;Liang, Yu-Jie;Wu, Xue;Guan, Wei;Xiao, Wen-Jing;...

通讯作者：

Xiao, Wen-Jing(wxiao@mail.ccnu.edu.cn);Chen, Jia-Rong(chenjiarong@mail.ccnu.edu.cn);Guan, Wei(guanw580@nenu.edu.cn)

作者机构：

[Wu, Xue; Xiao, Wen-Jing; Chen, Jia-Rong; Wang, Peng-Zi] Cent China Normal Univ, Coll Chem, CCNU uOttawa Joint Res Ctr, Key Lab Pesticides & Chem Biol,Minist Educ, Wuhan 430079, Hubei, Peoples R China.

[Liang, Yu-Jie; Guan, Wei] Northeast Normal Univ, Inst Funct Mat Chem, Fac Chem, Changchun 130024, Peoples R China.

[Xiao, Wen-Jing] Lanzhou Univ, State Key Lab Appl Organ Chem, Lanzhou 730000, Peoples R China.

[Chen, Jia-Rong] Henan Normal Univ, Sch Chem & Chem Engn, Xinxiang 453007, Henan, Peoples R China.

通讯机构：

[Wei Guan] I

[Wen-Jing Xiao; Jia-Rong Chen] C

CCNU-uOttawa Joint Research Centre, Key Laboratory of Pesticides & Chemical Biology Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079, China<&wdkj&>State Key Laboratory of Applied Organic Chemistry, Lanzhou University, Lanzhou 730000, P. R. China<&wdkj&>CCNU-uOttawa Joint Research Centre, Key Laboratory of Pesticides & Chemical Biology Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079, China<&wdkj&>School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang, Henan 453007, China<&wdkj&>Institute of Functional Material Chemistry, Faculty of Chemistry, Northeast Normal University, Changchun 130024, P. R. China

语种：

英文

关键词：

photocatalysis;copper catalysis;C-O coupling;alkene carbo-esterfication;photo-ATRA-type reaction

期刊：

ACS CATALYSIS

ISSN：

2155-5435

年：

2022

卷：

期：

页码：

10925-10937

DOI：

10.1021/acscatal.2c03576

基金类别：

National Natural Science Foundation of China [22171099, 21971081, 21820102003, 91956201, 21901080, 21773025]; Open Research Fund of School of Chemistry and Chemical Engineering, Henan Normal University [2021YB02]; Program of Introducing Talents of Discipline to Universities of China (111 Program) [B17019]; Excellent Doctoral Dissertation Cultivation Grant from CCNU [2022YBZZ003]

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

Atom transfer radical addition (ATRA) reaction of alkenes has had a significant impact on the field of radical difunctionalization of alkenes. Particularly, in the three-component photo-ATRA-type processes, a rich chemical space and structural diversity could be achieved by smart combination of redox-active radical precursors and the third coupling components (e.g., halides, C-, N-, and O-nucleophiles) under mild conditions. However, the inherent complicated mechanisms involving radical chain or outer-sphere SET of the incipient radical interme...

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Copper-Catalyzed Three-Component Photo-ATRA-Type Reaction for Asymmetric Intermolecular C-O Coupling

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