Photoinduced Cobalt Catalyzed Radical Heck-Type Reaction of Alkyl Electrophiles

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成果类型：

期刊论文

作者：

Gou, Shijia;Li, Chenyue;Liang, Tiantian;Peng, Chengyi;Bao, Feng*;...

通讯作者：

Bao, Feng;Ye, F;Wu, CG

作者机构：

[Ye, Fei; Liang, Tiantian; Peng, Chengyi; Gou, Shijia; Bao, Feng] Cent China Normal Univ, CCNU uOttawa Joint Res Ctr, Key Lab Pesticide & Chem Biol, Minist Educ,Coll Chem, Wuhan 430079, Hubei, Peoples R China.

[Li, Chenyue; Wu, Chenggui; Wu, CG] Minist Educ, Key Lab Xinan Med, Hefei 230038, Anhui, Peoples R China.

[Ye, Fei] Wuhan Inst Photochem & Technol, Wuhan 430082, Hubei, Peoples R China.

通讯机构：

[Ye, F ; Bao, F] C

[Wu, CG ] M

Cent China Normal Univ, CCNU uOttawa Joint Res Ctr, Key Lab Pesticide & Chem Biol, Minist Educ,Coll Chem, Wuhan 430079, Hubei, Peoples R China.

Minist Educ, Key Lab Xinan Med, Hefei 230038, Anhui, Peoples R China.

Wuhan Inst Photochem & Technol, Wuhan 430082, Hubei, Peoples R China.

语种：

英文

期刊：

Organic Letters

ISSN：

1523-7060

年：

2023

卷：

期：

页码：

8883-8888

DOI：

10.1021/acs.orglett.3c03676

基金类别：

Central China Normal University [22201088]; National Natural Science Foundation of China; Central China Normal University (CCNU)

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

We report here a general alkylation reaction of terminal alkenes with nucleophilic cobaloxime complex catalysis under visible light irradiation. A broad range of vinyl arenes and heteroarenes, as well as a diverse set of alkyl(pseudo)halides or strained rings as alkyl electrophiles, can efficiently undergo the transformation up to the gram scale. Mechanistic study reveals the radical nature of the reaction and corroborates our design involv...

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Photoinduced Cobalt Catalyzed Radical Heck-Type Reaction of Alkyl Electrophiles

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