Solar-Driven Water-Gas Shift Reaction over CuOx/Al2O3 with 1.1% of Light-to-Energy Storage

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成果类型：

期刊论文

作者：

Zhao, Likuan;Qi, Yuhang;Song, Lizhu;Ning, Shangbo;Ouyang, Shuxin*;...

通讯作者：

Ouyang, Shuxin

作者机构：

[Qi, Yuhang; Ning, Shangbo; Ye, Jinhua; Zhao, Likuan; Song, Lizhu; Ouyang, Shuxin] Tianjin Univ, TJU NIMS Int Collaborat Lab, Sch Mat Sci & Engn, 92 Weijin Rd, Tianjin 300072, Peoples R China.

[Ouyang, Shuxin] Cent China Normal Univ, Coll Chem, 152 Luoyu Rd, Wuhan 430079, Hubei, Peoples R China.

[Xu, Hua] Wuhan Inst Technol, Sch Chem & Environm Engn, 206 Guangguyi Rd, Wuhan 430205, Hubei, Peoples R China.

[Ye, Jinhua] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton WPI MANA, 1-1 Namiki, Tsukuba, Ibaraki 3050047, Japan.

通讯机构：

[Ouyang, Shuxin] T

[Ouyang, Shuxin] C

Tianjin Univ, TJU NIMS Int Collaborat Lab, Sch Mat Sci & Engn, 92 Weijin Rd, Tianjin 300072, Peoples R China.

Cent China Normal Univ, Coll Chem, 152 Luoyu Rd, Wuhan 430079, Hubei, Peoples R China.

语种：

英文

关键词：

CuOx;oxygen vacancy;photocatalysis;photothermal catalysis;water-gas shift (WGS) reaction

期刊：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN：

1433-7851

年：

2019

卷：

期：

页码：

7708-7712

DOI：

10.1002/anie.201902324

基金类别：

This work received financial support from the National Natural Science Foundation of China (Grants 21573158, 51502200, 51502198 and 21633004).

机构署名：

本校为通讯机构

院系归属：

化学学院

摘要：

Hydrogen production from coal gasification provides a cleaning approach to convert coal resource into chemical energy, but the key procedures of coal gasification and thermal catalytic water-gas shift (WGS) reaction in this energy technology still suffer from high energy cost. We herein propose adopting a solar-driven WGS process instead of traditional thermal catalysis, with the aim of greatly decreasing the energy consumption. Under light irradiation, the CuOx /Al2 O3 delivers excellent catalytic activity (122 mumol gcat (-1) s(-1) of H2 evolution and >95 % of CO conversion) which is even mo...

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Solar-Driven Water-Gas Shift Reaction over CuOx/Al2O3 with 1.1% of Light-to-Energy Storage

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