Designed Synthesis of Fe/Zr Bimetallic Organic Framework to Enhance the Selective Conversion of H2S to Sulfur - 成果

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Designed Synthesis of Fe/Zr Bimetallic Organic Framework to Enhance the Selective Conversion of H₂S to Sulfur

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成果类型：

期刊论文

作者：

Zheng, Xiaoxiao;Chen, Xiaoping;Li, Xiaoqing;Zhu, Jide;Chen, Jipeng;...

通讯作者：

Xu, YL;Shen, LJ

作者机构：

[Lin, Fengcai; Li, Xiaoqing; Zhu, Jide; Zheng, Xiaoxiao; Xu, Yanlian; Chen, Jipeng; Xu, YL] Minjiang Univ, Coll Mat & Chem Engn, Fujian Engn Res Ctr New Chinese Lacquer Mat, Fuzhou 350108, Fujian, Peoples R China.

[Shen, Lijuan; Shen, LJ; Zhu, Jide; Zheng, Xiaoxiao; Chen, Xiaoping; Jiang, Lilong] Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Fuzhou 350002, Fujian, Peoples R China.

[Chen, Xiaoping] Cent China Normal Univ, Inst Environm & Appl Chem, Coll Chem, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Hubei, Peoples R China.

[Shen, Lijuan; Shen, LJ] Fujian Normal Univ, Coll Environm & Resource Sci, Coll Carbon Neutral Modern Ind, Fujian Key Lab Pollut Control & Resource Reuse, Fuzhou 350007, Fujian, Peoples R China.

通讯机构：

[Shen, LJ ] F

[Xu, YL ] M

Minjiang Univ, Coll Mat & Chem Engn, Fujian Engn Res Ctr New Chinese Lacquer Mat, Fuzhou 350108, Fujian, Peoples R China.

Fuzhou Univ, Natl Engn Res Ctr Chem Fertilizer Catalyst, Fuzhou 350002, Fujian, Peoples R China.

Fujian Normal Univ, Coll Environm & Resource Sci, Coll Carbon Neutral Modern Ind, Fujian Key Lab Pollut Control & Resource Reuse, Fuzhou 350007, Fujian, Peoples R China.

语种：

英文

期刊：

INORGANIC CHEMISTRY

ISSN：

0020-1669

年：

2024

卷：

期：

页码：

5586-5597

DOI：

10.1021/acs.inorgchem.3c04543

基金类别：

Natural Science Foundation of Fujian Province [22178057, 21978050, 32301539]; National Natural Science Foundation of China [2020H6029]; Fujian Province Science and Technology Project: School-Enterprise Cooperation in Science and Engineering [FUHJF-L-2022-22]; Marine Economic Development Special Fund Project of Fujian Province [2022J05234, 2021J01197, 2022J011120, 2023J011574]; Natural Science Foundation of Fujian Province

机构署名：

本校为其他机构

院系归属：

化学学院

摘要：

The development of stable and effective catalysts to convert toxic H(2)S into high value-added sulfur is essential for production safety and environmental protection. However, the inherent defects of traditional iron- and zirconium-based catalysts, such as poor activity, high oxygen consumption, and low sulfur selectivity, limit their further developments and applications. Herein, the Fe-Zr bimetallic organic framework FeUIO-66(x) with different cubic morphologies was synthesized via a facile solvothermal method. The results indicate that the introduction of Fe not only increases the specific ...

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Designed Synthesis of Fe/Zr Bimetallic Organic Framework to Enhance the Selective Conversion of H₂S to Sulfur

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