PdBi Single-Atom Alloy Aerogels for Efficient Ethanol Oxidation

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成果类型：

期刊论文

作者：

Wang, Hengjia;Jiao, Lei;Zheng, Lirong;Fang, Qie;Qin, Ying;...

通讯作者：

Zhu, Chengzhou(czzhu@mail.ccnu.edu.cn);Wen, Jing(jing.wen@wit.edu.cn)

作者机构：

[Fang, Qie; Qin, Ying; Zhu, Chengzhou; Wei, Xiaoqian; Jiao, Lei; Luo, Xin; Gu, Wenling; Wang, Hengjia] Cent China Normal Univ, Coll Chem, Int Joint Res Ctr Intelligent Biosensing Technol, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

[Zheng, Lirong] Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China.

[Hu, Liuyong; Wen, Jing] Wuhan Inst Technol, Sch Mat Sci & Engn, Wuhan 430205, Peoples R China.

通讯机构：

[Jing Wen] S

[Chengzhou Zhu] K

Key Laboratory of Pesticide and Chemical Biology of Ministry of Education, International Joint Research Center for Intelligent Biosensing Technology and Health, College of Chemistry, Central China Normal University, Wuhan, 430079 P. R. China<&wdkj&>School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan, 430205 P. R. China

语种：

英文

关键词：

aerogels;electrocatalysis;ethanol oxidation reaction;self-assembly;single-atom alloys

期刊：

Advanced Functional Materials

ISSN：

1616-301X

年：

2021

卷：

期：

页码：

2103465-

DOI：

10.1002/adfm.202103465

基金类别：

The authors gratefully acknowledge the financial support by National Natural Science Foundation of China (nos. 22074049 and 22004042), self‐determined research funds of CCNU from the colleges’ basic research and operation of MOE (CCNU20QN007, CCNU20TS013), and the Program of Introducing Talents of Discipline to Universities of China (111 program, B17019). This work was carried out with the support of 1W1B beamline at the Beijing Synchrotron Radiation Facility.

机构署名：

本校为第一机构

院系归属：

化学学院

摘要：

Single-atom alloys (SAAs) have ignited a surge of unprecedented interest as the advanced nanomaterials and opened many opportunities for wide applications. Herein, 3D porous aerogels comprising ionic liquid (IL) functionalized PdBi SAA building blocks with atomically dispersed Bi on Pd nanowires (IL/Pd50Bi1) are synthesized with accelerated gelation kinetics, which could serve as high-efficiency electrocatalysts for ethanol oxidation reaction (EOR). Benefiting from the unique structures of aerogels including synergistic effects of PdBi SAA nano...

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PdBi Single-Atom Alloy Aerogels for Efficient Ethanol Oxidation

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