Photoredox-Enabled Chromium-Catalyzed Alkene Diacylations

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成果类型：

期刊论文

作者：

Liu, Jing;Lu, Liang-Qiu;Luo, Yixin;Zhao, Wei;Sun, Peng-Chao;...

通讯作者：

Cheng, Ying;Xiao, Wen-Jing;Qi, Xiaotian

作者机构：

[Zhao, Wei; Cheng, Ying; Lu, Liang-Qiu; Liu, Jing; Xiao, Wen-Jing; Xiao, WJ] Cent China Normal Univ, Coll Chem, CCNU uOttawa Joint Res Ctr, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

[Lu, Liang-Qiu] Chinese Acad Sci, Lanzhou Inst Chem Phys LICP, State Key Lab Oxo Synth & Select Oxidat, Lanzhou 730000, Peoples R China.

[Qi, Xiaotian; Luo, Yixin; Qi, XT] Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China.

[Sun, Peng-Chao; Jin, Weiwei] Xinjiang Univ, Coll Chem,Urumqi Key Lab Green Catalysis & Synth, State Key Lab Chem & Utilizat Carbon Based Energy, Key Lab Oil & Gas Fine Chem,Minist Educ & Xinjian, Urumqi 830046, Peoples R China.

通讯机构：

[Cheng, Y; Xiao, WJ ] C

[Qi, XT ] W

Cent China Normal Univ, Coll Chem, CCNU uOttawa Joint Res Ctr, Key Lab Pesticide & Chem Biol,Minist Educ, Wuhan 430079, Peoples R China.

Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China.

语种：

英文

关键词：

visible light;photoredox;chromium catalysis;alkene diacylations;diones

期刊：

ACS CATALYSIS

ISSN：

2155-5435

年：

2022

卷：

期：

页码：

1879-1885

DOI：

10.1021/acscatal.1c05672

基金类别：

National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [21822103, 21820102003, 21772052, 91956201, 21901080]; Program of Introducing Talents of Discipline to Universities of China (111 Program) [B17019]; Natural Science Foundation of the Hubei ProvinceNatural Science Foundation of Hubei Province [2017AHB047]; self-determined research funds of CCNU from the colleges' basic research and operation of MOE [CCNU20QN006]

机构署名：

本校为第一且通讯机构

院系归属：

化学学院

摘要：

Transition-metal-catalyzed cross-coupling reactions are a powerful tool to construct carbon-carbon bonds in modern synthetic chemistry. Chromium catalysis is much less developed compared with the widely used palladium and nickel catalysis. Herein, we reported an efficient and flexible chromium-catalyzed radical diacylation of alkenes with the help of visible-light photoredox catalysis, giving access to valuable 1,4-, 1,6-, and 1,7-diones under mild conditions. The synthetic utility of this methodology was proven by converting diones to diverse ...

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Photoredox-Enabled Chromium-Catalyzed Alkene Diacylations

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