Achieving In Situ Dynamic Fluorescence in the Solid State through Synergizing Cavities of Macrocycle and Channels of Framework

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成果类型：

期刊论文

作者：

He, Xuan;Tao, Wei;Zhang, Jing-Xuan;Wang, Tao;Shen, Dengke;...

通讯作者：

Zhang, Zhihan(zhihanzhang@ccnu.edu.cn);Wei, Peifa(pfwei@ahu.edu.cn)

作者机构：

[He, Xuan; Tao, Wei; Wei, Peifa; Wang, Tao; Shen, Dengke] Anhui Univ, Inst Phys Sci & Informat Technol, Anhui Graphene Engn Lab, Key Lab Struct & Funct Regulat Hybrid Mat,Minist E, Hefei 230039, Peoples R China.

[Zhang, Jing-Xuan] Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Guangdong, Peoples R China.

[Zhang, Zhihan] Cent China Normal Univ, Key Lab Pesticide & Chem Biol, CCNU uOttawa Joint Res Ctr, Coll Chem,Minist Educ, Wuhan 430079, Hubei, Peoples R China.

通讯机构：

[Zhihan Zhang] C

[Peifa Wei] A

Anhui Graphene Engineering Laboratory, Key Laboratory of Structure and Functional Regulation of Hybrid Materials of Ministry of Education, Institutes of Physical Science and Information Technology, Anhui University, Hefei 230039, China<&wdkj&>CCNU-uOttawa Joint Research Centre, Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079, China

语种：

英文

期刊：

ACS Materials Letters

ISSN：

2639-4979

年：

2023

卷：

期：

页码：

1227-1236

DOI：

10.1021/acsmaterialslett.2c01199

基金类别：

National Natural Science Foundation of China [22001006]; Open Project of Key Laboratory of Structure and Functional Regulation of Hybrid Materials of Anhui University, Ministry of Education

机构署名：

本校为其他机构

院系归属：

化学学院

摘要：

To achieve in situ dynamic fluorescence in the solid state and unveil the mechanism remain a formidable challenge. Herein, through synergizing the cavities of macrocycles for dynamic complexing and the channels of frameworks for facile transit, we construct intrinsic channels from an emissive cyclophane and realize precisely tunable emission in the solid state through the sequential guests’ exchange. Specifically, two design criteria involve (1) The twisted cyanostilbene units not only endow the systems with solid-state fluorescence but also t...

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Achieving In Situ Dynamic Fluorescence in the Solid State through Synergizing Cavities of Macrocycle and Channels of Framework

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