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Ultrafast Macroscopic Assembly of High-Strength Graphene Oxide Membranes by Implanting an Interlaminar Superhydrophilic Aisle

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成果类型:
期刊论文
作者:
Wang, Zhe;Mao, Boyang;Zhao, Ming;Calatayud, David G.;Qian, Wei;...
通讯作者:
He, DP;Kou, ZK
作者机构:
[Wang, Zhe; Zhao, Xin; Qian, Wei; Yan, Shilin; He, DP; He, Daping; Li, Peng] Wuhan Univ Technol, Sch Sci, Wuhan 430070, Peoples R China.
[Hu, Zhigang; Mao, Boyang] Univ Cambridge, Dept Engn, Cambridge CB3 0FA, England.
[Zhao, Ming] Cent China Normal Univ, Minist Educ, Coll Chem, Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China.
[Calatayud, David G.] Inst Ceram & Vidrio CSIC, Dept Electroceram, Madrid 28049, Spain.
[Kou, ZK; Kou, Zongkui; Fu, Huaqiang] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China.
通讯机构:
[Kou, ZK ; He, DP ] W
Wuhan Univ Technol, Sch Sci, Wuhan 430070, Peoples R China.
Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China.
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Peoples R China.
语种:
英文
关键词:
graphene oxide;membranes;ultrafast macroscopic assembly;strength;superhydrophilic aisle
期刊:
ACS Nano
ISSN:
1936-0851
年:
2022
卷:
16
期:
3
页码:
3934-3942
基金类别:
The authors acknowledge financial support from the National Natural Science Foundation of China (51672204), the Fundamental Research Funds for the Central Universities (WUT: 2020IB005), 2018 National Key R&D Program of China (257), Foundation of National Key Laboratory on Electromagnetic Environment Effects (No. 614220504030617), and ComFuturo Program second Edition-Fundacion General CSIC. The authors also acknowledge the Center for Materials Research and Analysis at the Wuhan University of Technology for the TEM and image suggestions from Dr. Xiaoqing Liu.
机构署名:
本校为其他机构
院系归属:
化学学院
摘要:
A macroscopic-assembled graphene oxide (GO) membrane with sustainable high strength presents a bright future for its applications in ionic and molecular filtration for water purification or fast force response for sensors. Traditionally, the bottom-up macroscopic assembly of GO sheets is optimized by widening the interlaminar space for expediting water passage, frequently leading to a compromise in strength, assembly time, and ensemble thickness. Herein, we rationalize this strategy by implanting a superhydrophilic bridge of cobalt-based metal-...

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