Engineering the Redox-Driven Channel for Precisely Regulating Nanoconfined Glutathione Identification and Transport

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成果类型：

期刊论文

作者：

Guan, Tianpei;Cheng, Ming;Zeng, Lisi;Chen, Xiaoya;Xie, Yuan;...

通讯作者：

Wang, Jin;Cui, Shuzhong;Sun, Yao;Li, Haibing

作者机构：

[Lei, Ziying; Wang, Jin; Cui, SZ; Guan, Tianpei; Ruan, Qiang; Cui, Shuzhong; Zeng, Lisi] Guangzhou Med Univ, Dept Gastroentestinal Surg 2, Affiliated Canc Hosp & Inst, Guangzhou 510095, Peoples R China.

[Chen, Xiaoya; Sun, Yao; Sun, Y; Li, Haibing; Cheng, Ming] Cent China Normal Univ, Coll Chem, Key Lab Pesticide & Chem Biol CCNU, Minist Educ, Wuhan 430079, Peoples R China.

[Xie, Yuan] Guangdong Prov Key Lab Radioact & Rare Resource U, Shaoguan 512026, Peoples R China.

通讯机构：

[Wang, J; Cui, SZ] G

[Sun, Y; Li, HB] C

Guangzhou Med Univ, Dept Gastroentestinal Surg 2, Affiliated Canc Hosp & Inst, Guangzhou 510095, Peoples R China.

Cent China Normal Univ, Coll Chem, Key Lab Pesticide & Chem Biol CCNU, Minist Educ, Wuhan 430079, Peoples R China.

语种：

英文

关键词：

artificial intelligent nanochannel;glutathione;host−guest;redox-regulated switch;selective transport

期刊：

ACS Applied Materials & Interfaces

ISSN：

1944-8244

年：

2021

卷：

期：

页码：

49137-49145

DOI：

10.1021/acsami.1c12061

基金类别：

NSFCNational Natural Science Foundation of China (NSFC) [22022404, 22074050, 21772055, 21572076, 81972918]; Postdoctoral Science Foundation of ChinaChina Postdoctoral Science Foundation [2019M652852, 2020M672388]; Guangdong Major Clinical Technology Program [2019ZD16]; Research Fund Program of the Guangdong Key Laboratory of Radioactive and Rare Resource Utilization [2018B030322009]

机构署名：

本校为通讯机构

院系归属：

化学学院

摘要：

Bioinspired artificial nanochannels for molecular and ionic transport have extensive applications. However, it is still a huge challenge to achieve an intelligent transport system with high selectivity/efficiency and controllability. Inspired by glutathione transport across the plasma membrane via redox regulation, we herein designed and fabricated a redox-reactive artificial nanochannel based on the host-guest chemical strategy. The nanochannel platform achieved high selectivity/efficiency for the identification and transmission of glutathione...

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Engineering the Redox-Driven Channel for Precisely Regulating Nanoconfined Glutathione Identification and Transport

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